1. Field of the Invention
This invention relates generally to small neutron sources and more specifically to bright thermal neutron beam production from compact sources including neutron energy moderators.
2. Description of the Related Art
Non-Destructive Testing (NDT) of structures through imaging of internal structural parts is a known examination procedure and is continuing to be further developed in ever expanding business arenas. Imaging of internal parts or portions of structures using x-rays and y-rays is a multibillion dollar business. Not yet well developed, though, is NDT imaging using neutrons, i.e., neutron radiography.
This situation arises because practical, small and relatively portable thermal neutron sources that provide bright or intense beams of thermal neutrons have not been available. Bright or intense neutron beams have a large number of neutrons per second passing through a defined area, i.e., n/sec-cm2. To date, neutron radiography primarily has been done in laboratories using thermal neutrons, i.e., about 0.025 electron-volt (eV) energy neutrons, provided from nuclear reactors. Clearly, nuclear reactors are complex, and both extremely costly and large. Use of nuclear reactors as thermal neutron sources limits industrial applications. These laboratory experiments, however, have demonstrated the potential industrial utility of neutron radiography, but implementation of practical industrial applications has been restricted by the unavailability of small, portable sources of bright, thermal neutron beams.
Currently available portable neutron sources include isotope material sources, that use neutron producing radio isotopes such as Californium (Cf 252). These radio isotope sources fail as practical thermal neutron sources for neutron radiography because of their low neutron output and in particular because they produce neutrons in all directions that preclude outputting bright narrow neutron beams. Further, radio isotope sources raise safety issues and logistical complications. For example, concerns have increased recently about the physical security of radio isotope sources because of their possible use in dirty bombs.
Also currently available as neutron sources are systems using ion beams to produce deuterium (D)-tritium (T), D-D or T-T reactions. Neutrons produced by such reactions, however, have energies that must be attenuated in order to be at thermal energy levels. To slow produced neutrons down to thermal energies requires passage of the neutrons through a moderator material. Known moderator material arrangements involve arrangement of moderator material about a primary neutron source where the D-D, D-T or T-T reactions occur and produce fast neutrons in all directions. Accordingly such primary neutron source and moderator arrangements are quite large in size. Since the reaction produced fast neutrons are emitted in all directions, the large exterior surface of the area of the arranged moderator material determines the minimal source size. Many neutron radiography applications require high brightness thermal neutron sources, and when oversized sources with their low brightness emitted neutron beams are used the resulting radiography images have intrinsically lowered resolution.
Currently known neutron radiography applications among many others that could use small bright thermal neutron sources include: NDT at nuclear power plants; NDT for aircraft inspection; and, boron neutron capture cancer therapy.
To assure safe operation of nuclear power plants, the rates of corrosion at critical locations must be monitored along with the integrity of critical system components such as reactor coolant pump seals. Neutron radiography could be used to provide such monitoring if effective portable bright neutron sources were available, and, thereby, greatly reduce maintenance costs and unscheduled downtime. Other inspections that neutron radiography could be used for include: detection and characterization of material fractures and crack growth; and, examinations of inaccessible and otherwise unobservable structures such as metallic pressure boundaries. Neutron radiography not only could provide significant operation and maintenance cost savings, but also could improve structural integrity assessments and estimates of critical machinery and component remaining lifetimes. Thereby, providing for more accurate planning for nuclear reactor maintenance outages and in-service inspections.
Commercial, military and private aircraft are being used for increasingly longer lifetimes, and thus require more accurate and involved inspections. Neutron radiography is ideal, for example, in detecting and monitoring corrosion of aircraft structural components. Neutron radiography also is ideal for inspecting structures such as piping and conduits enclosed in multiple layers of extended insulation materials. Other inspection techniques for these situations such as ultrasonic inspections are ineffective or impossible to apply. Information on the state and location of corrosion can be precisely provided using neutron radiography, whereas the same detail of information would not be available using x-ray inspection. Canadian studies have shown that neutron radiography is the only inspection method that can detect small areas of moisture entrapment and corrosion (W. J Lewis, L. G. I. Bennett, “Moisture and Corrosion Inspection of Aircraft Composite Flight Controls with Neutron Radiography,” 1998 ASNT Spring Conference, Anaheim, Calif.). Neutron computer tomography already is a leading technology used to detect excessive hydration levels that cause titanium jet engine fan blade embrittlement. Neutron radiography also has been used to provide real time imaging of fluid movements in running engines and hydraulic systems to detect voids and other problems.
A non-imaging neutron application where a portable, small bright thermal neutron source could be of significant potential is in the field of medicine. Specifically, such an application is Boron Neutron Capture Therapy (BNCT). Possible applications for BNCT include treatment of brain and liver cancer, and arthritis. The BNCT procedures involve injecting boron-containing compounds into a patient that then accumulate in malignant tumors. A beam of thermal neutrons is directed at the patient to irradiate the malignant tumors where boron atoms preferentially capture neutrons. After capturing neutrons, the excited boron nuclei decay to release short-range radiation (alpha particles). This short-range radiation destroys nearby tumor tissue, but does not travel far enough to damage non-tumor surrounding tissue. To date, nuclear reactors and accelerators, which are large and expensive and are inappropriate for clinical settings, have been used to provide thermal neutrons for BNCT experiments and procedures. The lack of small, convenient, bright, thermal neutron sources has been a major obstacle to acceptance and use of BNCT.
Another non-imaging neutron application where a compact thermal neutron source could be of significant potential is in the field of material analysis, which has to date been generally relegated to large national laboratories due to the historical dependence for the analysis upon nuclear reactors. These techniques, e.g., Prompt Gamma Neutron Activation Analysis (PGNAA). Short-Lived Neutron Activation Analysis (SLNAA), and Neutron Activation Analysis (NAA), could be developed for field use and small laboratory use, if a compact thermal neutron generator could be manufactured, thus severing the ‘umbilical cord’ to nuclear reactors. Combining a PGNAA/SLNAA detection system with a compact thermal-neutron generator has the potential to revolutionize both qualitative and quantitative assays of most inorganic chemicals and certain hetero-organic compounds. All elements from hydrogen up to the highest-Z actinide can be assayed simultaneously with high specificity, quality and, in many cases, sensitivity using neutrons.
The non-destructive nature of PGNAA, SLNAA and NAA, and the penetrating qualities of neutrons offer a unique approach toward the study, for example, of manufacturing-induced metallurgical anomalies in structural materials, chemical anomalies in semiconductor materials, and geological phenomena. There would also be direct applications for portable bright neutron sources to many applications such as Homeland Security issues for the detection of nerve agents and explosives. Also, applications would include the chemical and semiconductor industries, in-field metallurgical evaluations, the characterization of legacy and/or hazardous materials, forensics, the analysis of archaeological artifacts, geological analysis, the detection of land mines, etc. The relative novelty of a portable bright neutron source offers many options to educational institutes that have a strong interest and background in many of the above-cited fields. Internationally, a portable bright neutron source will permit countries to have capabilities to detect and interdict the unauthorized movement of explosives, nerve agents, nuclear, other radioactive materials and also other hazardous materials.
Prior encountered problems where intense thermal neutron beams could be used are overcome using a compact ion source with a target where reactions occur to produce fast neutrons that are lowered in energy to thermal neutron levels using moderator materials. Two or more stages of moderator materials can be used for the described thermal neutron source.
The first stage of moderator material is positioned as close as possible to the target. It can be positioned either: (1) about a secondary electron shield that is located close to the target where fast neutrons are produced; or, (2) under a target for both cooling the target and moderating generated fast neutrons. This first stage moderator can be: (1) a layer of water contained in a target shroud having the secondary electron shield as the inner wall; or, (2) a layer of water directly below the target.
The second stage of moderator is positioned about the first stage moderator. The second stage moderator can be made of polyethylene or lead-loaded polyethylene.
A thermal neutron port is positioned through the second stage moderator to provide for a produced thermal neutron ion exit. This thermal neutron port can be cone shaped with a large base of the cone positioned to face the first stage moderator and a small cone apex positioned to output thermal neutrons.
A further advantage of the disclosed compact thermal neutron source is that alternative to outputting thermal neutrons, the disclosed neutron source also can output fast neutrons along a source longitudinal axis.
Aspects of the present invention are described herein in the context of a compact neutron generator including two-stages of neutron moderators to produce a bright thermal neutron beam. Those of ordinary skill in the art will realize that the following detailed description of the present invention is illustrative only and is not intended to be in any way limiting. Other aspects of the present invention will readily suggest themselves to such skilled persons having the benefit of this disclosure. Reference will now be made in detail to implementations of the present invention illustrated in the accompanying drawings. The same reference indicators will be used throughout the drawings and the following detailed description to refer to the same or like parts.
In the interest of clarity, not all of the routine features of the implementations described herein are shown and described. It will, of course, be appreciated that in the development of any such actual implementation, numerous implementation—specific decisions must be made in order to achieve the developer's specific goals, such as compliance with application—and business-related constraints, and that these specific goals will vary from one implementation to another and from one developer to another. Moreover, it will be appreciated that such a development effort might be complex and time-consuming, but would nevertheless be a routine undertaking of engineering for those of ordinary skill in the art having the benefit of this disclosure.
The new compact thermal neutron source, designated with the general numeral 10, consists of a Radio Frequency (RF) antenna 12 to power an ion source 14 that emits ions toward a target 16 from which neutrons are emitted because of reactions between incoming ions and ions that previously impacted the target 16. The previously impacted ions are loaded onto the target 16. Types of ions that can be used for these reactions include deuterium-2H (D) or tritium-3H (T). Deuterium-deuterium (D-D) reactions and deuterium-tritium reactions both produce neutrons. The produced neutrons, however, are characterized as fast neutrons because of their about 2.5 to about 14.1 million electron-Volt (MeV) energies. These fast neutrons, after production, must somehow be moderated to thermal energy levels of about 0.025 eV in order for the produced neutrons to be thermal neutrons. Tritium-tritium (T-T) reactions also produce fast neutrons, but T-T reactions are not favored for many applications because of the required amounts of tritium which introduce serious radiation safety requirements.
The ion source 14 emits an intense beam of ions (about 10 milliampers (mA)) at accelerated speeds (about 100 kilvolts (kV)) toward the target 16 that can be a metal hydride material. A useful exterior target 16 coating material for having impacting deuterium or tritium ions loaded so they can be impacted by other deuterium or tritium ions to react is titanium (Ti). Other useful target coating materials or target materials for effecting neutron producing reactions also are known to those skilled in the art. As discussed above the resulting fast neutrons are produced in all directions, i.e., 4 π steradians (str).
Positioned between the ion source 14 and the target 16 is a secondary electron shield 18 with an ion entrance aperture 20 (see
To moderate produced fast neutrons to thermal energies, the compact thermal neutron source 10 includes a first stage moderator 22 and a second stage moderator 24. First stage moderator 22 is positioned as proximate to target 16 where fast neutrons are produced as practical, and second stage moderator 24 is positioned as an exterior component of the compact thermal neutron source 10 as shown in
Accordingly, in an aspect for the invention, first stage moderator 22 is positioned inside vacuum envelope 26 of compact thermal neutron source 10.
An exit from compact thermal neutron source 10 for produced thermal neutrons is thermal neutron port 28. Assuring that enhanced thermal neutron fluxes are passed out through thermal neutron port 28 requires that first stage moderator 22 be arranged to substantially surround and be proximate to target 16. This arrangement and positioning of first stage moderator 22 ensures that essentially all produced fast neutrons pass through first stage moderator 22 and thereby have their energies reduced inside of vacuum envelope 26. Neutrons further can be slowed down and trapped near the vicinity of the first stage moderator 22 by surrounding the first stage moderator 22 with an additional neutron-absorbing material as a second stage moderator 24. Positioned through second stage moderator 24 is thermal neutron port 28. This thermal neutron port 28 is arranged in a cone shape with a large cone base being directed to be proximate to first stage moderator 22 as opposed to other smaller portions of the cone. This arrangement allows for more neutrons to enter the thermal neutron port 28 cone base from the interior of compact thermal neutron source 10 than would enter, for example, a cylindrical shaped thermal neutron port, and, thereby, more neutrons exit thermal neutron port 28 at the cone apex. To reduce risk of passing fast neutrons through thermal neutron port 28, the central axis 30 of thermal neutron port 28 (see
Polyethylene can be a material used for second stage moderator 24. This material moderates fast neutrons and also reflects thermal neutrons. Other neutron energy moderator and reflector materials that could be used for second stage moderator 24 are known to those skilled in the art, and can be so used for second stage moderator 24. For a preferred aspect of the invention, second stage moderator 24 is about 10-40 cm thick. Such an arrangement and sizing of second stage moderator 24 allows cylindrically symmetric side and backscattered neutrons to be directed toward thermal neutron port 28. This sizing and arrangement with respect to target 16 also maximizes elastic and inelastic neutron interactions to increase the potential for forward scattering of thermal energy neutrons toward thermal neutron port 28. A third stage of moderation that surrounds the second stage of moderation can be included to reflect neutrons back into the first and second stages of moderation (e.g., see
Various configurations of compact thermal neutron source 10 for neutron beam shaping have been modeled in order to optimize thermal neutron beam outputs. This modeling was effected using a known Monte Carlo N-Particles (MCNP) computerized model. MCNP is a general-purpose software code used for neutron, photon, electron or coupled neutron/photon/electron transport analysis. The MCNP software code uses geometric cells to analyze arbitrary three-dimensional configurations of materials. For neutrons, all reactions given in a particular cross-section evaluation are accounted for using MCNP. Scattering of neutrons is described using a free gas model and tabulated thermal neutron scattering data, S (alpha, beta) treatment are available for some materials such as light water and beryllium.
MCNP permits a two plane, two dimensional, graphical input for a modeled compact thermal neutron source 10, including moderator/reflector geometries and materials. In the instance of one modeled embodiment, the compact thermal neutron source 10 had D-D reactions occurring within a 3 cm thick water first stage moderator 22 and a 5 cm thick lead (Pb) loaded polyethylene second stage moderator 24. This modeled arrangement is shown in
The compact thermal neutron source 10 also is capable of being arranged to supply both fast and thermal neutrons. Supply of fast neutrons is along the compact thermal neutron source 10 longitudinal axis 32 where first stage moderator 22 material is minimal. As discussed above, thermal neutron output from compact thermal neutron source 10 is perpendicular to longitudinal axis 32. Fast neutron output along longitudinal axis 32 can effectively occur through ion source 14, because ion source 14 is hollow and only slightly attenuates passing fast neutrons. A fast neutron collinator that consists of separated plates of fast neutron shielding materials (not shown) to collinate a fast neutron beam can be positioned outside of compact thermal neutron source 10. For the above described compact thermal neutron source 10, the produced fast neutron beam can be 1-3 millimeters (mm). The fast neutron intensity will be approximately 109 neutrons per second, and the fast neutron brightness will be on the order of 4×107 n/(sec-mm2-str).
Target 16 can be cooled using recirculated water. To facilitate flexibility and utility in the operation of compact thermal neutron source 10, the water supply for the first stage moderator 22 is provided as an independent supply from the water supply for cooling target 16.
These two water supplies, therefore, can be independently operated. This independence in water supplies provides for operator control of thermal neutron outputs. Specifically, if water is drained from first stage moderator 22, the output of thermal neutrons is minimized.
In another aspect, designated by the general numeral 70, and shown in
As in the case of the compact thermal neutron source 10 of
In another aspect for the invention, a compact thermal neutron source and sample system that are designated by the general numeral 82 is shown in
Those skilled in the art of Short-Lived Neutron Activation Analysis (SLNAA) and Neutron Activation Analysis (NAA) understand that the apparatus shown in
While embodiments and applications of this invention have been shown and described, it would be apparent to those skilled in the art having the benefit of this disclosure that many more modifications than mentioned above are possible without departing from the inventive concepts herein. The invention, therefore, is not to be restricted except in the spirit of the appended claims.
This application claims priority from Provisional Patent Application Ser. No. 60/812,114 filed Jun. 9, 2006, and this application incorporates by reference all subject matter contained in that provisional patent application.
This invention was made with government support under Contract No. DE-AC02-05CH 11231 awarded by the United States Department of Energy to The Regents of the University of California for management and operation of the Lawrence Berkeley National Laboratory. The government has certain rights in this invention.
Filing Document | Filing Date | Country | Kind | 371c Date |
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PCT/US07/13638 | 6/11/2007 | WO | 00 | 11/23/2009 |
Number | Date | Country | |
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60812114 | Jun 2006 | US |