The invention generally relates to a hollow fiber compression scheme for energetic femtosecond pulses.
More in detail, the invention concerns a device for increasing the spectral bandwidth of optical pulses, said device comprising
a hollow fiber waveguide having an input end and an output end,
optical components for focusing the beam into the hollow fiber waveguide and for re-collimating the beam at the output end of the hollow fiber waveguide,
the said hollow fiber waveguide being contained in an air-tight chamber filled with a gas at a given pressure,
the compact table-top device for increasing the spectral bandwidth of multi-mJ femtosecond pulses.
Furthermore, the invention is directed to an arrangement where such a device is used, and to a corresponding method, namely for reducing the duration of optical pulses.
Few-cycle intense femtosecond pulses are an important and an enabling tool in time-resolved spectroscopy measurements and particularly in attosecond physics. However, despite essential progress in the development of chirped pulse amplifiers (CPAs), in practice, the shortest pulses generated from such a source have only reached 15 femtoseconds (fs). This is to be traced back to a fundamental limitation, namely gain narrowing in the laser crystal that results in reduced spectral bandwidths, and consequently in increased pulse durations. Hollow fiber compression (HFC) allows to overcome this limitation by broadening the spectrum of the pulses generated with femtosecond amplifiers. The spectrally broadened pulses are subsequently compressed in a negative dispersion delay line.
HFC relies on the nonlinear propagation of intense femtosecond pulses in gas-filled capillary tubes.
In
According to these
Furthermore,
Self-phase-modulation in a hollow fiber waveguide leads to spectral broadening while the spatial filtering properties of the waveguide ensure a transversally homogeneous spectral broadening and result in an excellent beam profile. Initially devised for sub-mJ pulses (see for instance M. Nisoli et al., “A novel-high energy pulse compression system: generation of multigigawatt sub-5-fs pulses”, Appl. Phys. Lett. B 65 (1997): p. 189-196), the method enabled the generation of sub-TW few-cycle pulses at KHz repetition frequencies from table-top systems. Subsequently, CPAs equipped with HFCs became the working horse of many femto- and atto-second physics laboratories around the world. However, several applications including high-photon yield high order harmonic generation, the generation of high-photon energy harmonic radiation, or the investigation of relativistic laser field-matter interactions call for few-cycle driving laser pulses with energies in excess of 1 mJ. With CPAs supplying multi-mJ pulses with durations in the range of 30-50 fs widely available, energy up-scaling of pulse compressors gained paramount importance for the development of laser sources for strong-field physics. However, energy up-scaling of HFC is not trivial since several phenomena affect the performance of HFCs when the pulse energy is increased beyond 1 mJ, as for instance ionization of the propagation medium, damage of the fiber entrance, self-phase modulation and self-focusing in front of the fiber.
Light propagation in a hollow fiber waveguide can be described by decomposing the optical field in discrete spatial modes with transversal mode profiles given by
V
jp
=J
j(ujpr/a)
where
Jj with j=0,1, . . . is the Bessel function of order j;
ujp with p=1,2, . . . is the pth root of the equation Jj(ujp)=0;
r is the radial coordinate (in a cylindrical coordinates system having its symmetry axis collinear with the symmetry axis of the hollow fiber); and
a is the fiber radius (see
The longitudinally polarized (LP) modes having a spatial profile Vjp are dubbed the LPjp modes. The complex propagation constant kjp of the mode jp is given by
k
jp(ω)=βjp(ω)+iαjp(ω)
with
ω being the angular frequency of the laser light; and
βjp, αjp being the real, respectively imaginary parts of the propagation constant.
The modes thus have different attenuation constants αjp(ω)=2.814ujp/a3[λ/(2π)]2,
with
λ=wavelength of the laser light;
and this accounts for the spatial filtering properties of the fiber.
The mode LP01 exhibits the smallest propagation losses and is referred to as fundamental or lowest-order mode. This mode LP01 has a profile given by a first order Bessel function (compare also
In the presence of a nonlinear effect occurring during propagation in the waveguide (either the Kerr-effect or ionization), energy is coupled from the fundamental mode LP01 to higher-order modes (cf. G. Tempea and T. Brabec, “Theory of self-focusing in a hollow wa-waveguide”, Opt. Lett. 23 (10) (1998): p. 762-764) which might lead to a degradation of the beam profile. Given the extremely high losses and low coupling coefficients of modes with j>2, it is sufficient to consider only coupling to the mode LP02 for the analysis of this phenomenon. The difference between the real parts β01(ω) and β02(ω) of the propagation constants kjp of the modes LP01 and LP02 and between their first order derivatives (with respect to the angular frequency ω) leads to phase mismatch (i.e. the phase of the two modes changes at different rates during propagation), or to group velocity mismatch, respectively (the two modes propagate with different velocities) between the modes. These phenomena can be quantified by means of the following parameters: the phase-mismatch length Lp12 can be described as
L
p12=λ0/[4πa2(u022−u012)],
with
λ0=carrier wavelength of the pulse to be compressed
(Lp12 being equal to 2×10−6×a2 for a center wavelength λ0 of 800 nm) and is the propagation length required for a phase difference of π to build up between the phases of the modes LP01 and LP02; the group-velocity mismatch length Lv12 can be described as
L
v12=2τFWHMcLp12/λ0,
with
τFWHM=half maximum pulse duration; and
c=speed of light in vacuum,
and is the propagation length required for a delay equal to the full width at half maximum pulse duration τFWHM to build up between the modes LP01 and LP02.
The physical meaning of these two quantities is the following: energy is coupled from the mode LP01 and LP02 as long as the phase difference between the two modes is <π, i.e. for propagation length l<Lp12. Subsequently, energy is coupling back to the fundamental mode LP01 for propagation lengths LP12<l<2 LP12 and this process of periodic energy transfer between the modes LP01 and LP02 is repeated as long as there is still significant temporal overlapping between the pulses propagating with the two spatial modes, i.e. for lengths l<Lv12.
Corresponding to the three phenomena governing mode-coupled propagation (phase-mismatch, group velocity mismatch and mode-dependent losses), three regimes A, B, C of propagation can be identified:
(A) The Phase-Mismatched Periodic Mode-Coupling Propagation:
(B) Reduced-Coupling Propagation:
(C) De-Coupled Propagation:
Hollow fiber compression schemes proposed so far rely on the loss-related mode discrimination mechanism; the fiber length is chosen such that the transmittance of the mode LP02 is negligible as compared to the transmittance of the mode LP01 (see U.S. Pat. No. 5,956,173 A; and M. Nisoli et al., “A novel-high energy pulse compression system: generation of multigigawatt sub-5-fs pulses”, Appl. Phys. Lett. B 65 (1997): p. 189-196; in particular p. 190, FIG. 1b and the corresponding discussion at the end of section 1). This method is well applicable for the compression of pulses with energies of approximately 1 mJ and slightly beyond, where fibers with diameters up to 200 μm-300 μm can be used. Compression of more energetic pulses (with energies well beyond 1 mJ) calls for the use of fibers with larger diameters in order to avoid excessive nonlinearities and/or damage of the fiber entrance. However, the loss-related mode discrimination of the fiber decreases rapidly with increasing fiber radius a according to the formula:
(α01(ω)−α02(ω))=2.814(u01−u02)/a3[λ/(2π)]2
Consequently, very long fibers need to be used in order to achieve proper mode filtering. In order to compress 30 fs/5 mJ pulses to 5 fs/2.5 mJ pulses, in practical tests (S. Bohman et al., Opt. Express 16 (2008): p. 10684), a fiber with a diameter of 500 μm and having a length of 2.2 m was used. Additionally, a differentially pumped chamber (that was evacuated at the extremity where the pulses were coupled) had to be used in order to reduce nonlinear effects in front of the fiber, and therewith to reduce the energy coupled into the higher-order mode LP02 at the fiber entrance (input end). The differential-pumping scheme adds significant complexity to the setup, while the length of the HFC chamber alone was approximately 4 m, exceeding thus the size of a typical table-top setup.
It is now an object of the invention to provide a hollow fiber waveguide device as mentioned above with which it is possible to increase the spectral bandwidth of multi-mJ optical pulses, and this by having a compact, table-top layout of the device.
It is a further object of the invention to provide a hollow fiber compressor arrangement for reducing the duration of optical pulses which is capable of generating multi-mJ pulses with good beam profile.
Furthermore, it is an object of the invention to provide a corresponding method for reducing the duration of optical pulses in an efficient, yet comparably simple manner, that in addition ensures a good beam profile.
According to a first aspect, the invention provides a device for increasing the spectral bandwidth of optical pulses, said device comprising
a hollow fiber waveguide having an input end and an output end,
optical components for focusing the beam into the hollow fiber waveguide and for re-collimating the beam at the output end of the hollow fiber waveguide,
the hollow fiber waveguide being contained in an air-tight chamber filled with a gas at a given pressure,
wherein the length of the hollow fiber is such that, for a given input pulse energy and gas pressure, the energy contained in a fundamental propagation mode, LP01, of the optical pulses that has minimum propagation losses exhibits substantially periodic oscillations over the full length of the hollow fiber waveguide and reaches a local maximum at the output end of the said hollow fiber waveguide.
Preferably, the length of the hollow fiber wave-waveguide is substantially equal to an even integer multiple of a phase-mismatch length Lp12, with
L
p12=2×10−6×a2,
where
a is the radius of the hollow fiber waveguide.
Further, it is preferred that the length of the hollow fiber waveguide is shorter than a group velocity mismatch length Lv12, with
L
v12=2τFWHMcLp12/λ0=4×10−6τFWHMca2/λ0,
where
a is the radius of the hollow waveguide;
λ0 is the carrier wavelength of the pulse to be compressed;
τFWHM is the full width at half maximum duration of the pulse to be compressed; and
c is the speed of light in vacuum.
The hollow fiber waveguide may e.g. be made of fused silica or BK7 glass.
Furthermore, the hollow fiber waveguide may simply be a cylindrical tube.
To avoid damages to the input end of the hollow fiber waveguide due to beam-pointing drifts causing the beam to impinge on the cladding of the hollow fiber waveguide, it is preferred that the hollow fiber waveguide has a cylindrical section and a substantially conical section at the input end, the optical pulses being coupled into the conical input end of the hollow fiber waveguide; or that the hollow fiber waveguide has an axis of symmetry, and is cleaved under an angle different from 90° with respect to the axis of symmetry.
The hollow fiber waveguide may preferably be filled with one of the following gases: Xe, Kr, Ar, Ne, He, N2, air.
According to a second aspect, the invention provides an arrangement for reducing the duration of optical impulses, that arrangement comprising a device as defined above, and further comprising a group delay dispersion compensation device.
This group delay dispersion compensation device may, for instance, comprise one or more prism pairs; one or more grating pairs; grating pairs and prism pairs; most preferably dispersive mirrors; or dispersive mirrors and one or more prism pairs.
According to a third aspect, the invention provides a method for reducing the duration of optical pulses comprising the steps:
As already mentioned, the hollow fiber waveguide preferably has a cylindrical section, and has a conical section at the input end, the light being coupled in at the conical input end; here, it is particularly preferred that coupling of the optical pulses into the hollow fiber waveguide is achieved by focusing the beam to a diameter equal to 60-80% percent of the diameter of the cylindrical section of the hollow fiber waveguide; or that coupling of the optical pulses into the hollow fiber waveguide is achieved by focusing the beam to a diameter equal to 60-80% percent of the maximum diameter of the conical section of the hollow fiber waveguide.
The invention is described now in more detail with reference to preferred embodiments to which the invention, however, should not be limited, and on the basis of the accompanying drawings in which
First, with reference to
In
With reference to
Here, it may be reminded that it is an object of this invention to devise hollow fiber compressor means which are capable to generate multi-mJ pulses with a good beam profile, from a compact setup. Furthermore, as pointed out above, the approach relying on the difference in the transmittance of the fiber 3A for the modes LP01 and LP02 and on differentially pumped chambers fails to fulfill these requirements.
The solution here proposed draws on the periodic energy transfer between the modes LP01 and LP02 (corresponding to the above regime (A) of propagation) that takes place over distances that are much shorter than the length required to suppress the mode LP02 via losses, resulting thus in a much more compact setup, with substantially reduced fiber length Lf(
L
f=2*N*Lp12,Lf<Lv12,
where N is a positive integer number.
This type of behavior (predicted in G. Tempea and T. Brabec, “Theory of self-focusing in a hollow waveguide”, Opt. Lett. 23 (10) (1008): p. 762-764; by means of an approximate analytical model and confirmed by D. Homoelle and A. L. Gaeta, “Nonlinear propagation dynamics of an ultrashort pulse in a hollow waveguide”, Opt. Lett. 25 (10) (2000): p. 761-763; by means of a thorough numerical analysis) is qualitatively illustrated in
The approach here proposed results both in a better throughput for the fundamental mode LP01 and in shorter fiber lengths Lf leading to improved compactness.
With reference to
With the issue of compactness being such solved, one is still concerned with possible damage that might result from slight beam-pointing drifts causing the laser beam 1 to irradiate the cladding 9 of the hollow tube 3A at the entrance (input end). In the case of a conventional, cylindrical hollow waveguide (cf.
The laser light fluence on the entrance surface 11 (and therewith the risk of accidental damage) can be reduced by employing a tapered, i.e. conical fiber section 14 at the entrance of the fiber 3A, as shown in
4*tan2α
as compared to a standard (non-tapered, cleaved under normal angle) hollow fiber. As an example, for a taper angle α=5°, the fluence is reduced by a factor of 0.031.
The beam waist 15 can also be matched for optimal coupling into the conical section 14 of the fiber 3A, as depicted in
Alternatively, one can cleave the hollow waveguide 3 under an oblique angle β, as is shown in