The present disclosure is generally related to devices, systems, and methods for generating power using gamma ray sources, such as, for example, depleted cobalt-60 (Co-60) irradiators. The power generated using the devices, systems, and methods described herein can be in the form of electric power, heat, or a combination thereof.
The following summary is provided to facilitate an understanding of some of the innovative features unique to the aspects disclosed herein, and is not intended to be a full description. A full appreciation of the various aspects disclosed herein can be gained by taking the entire specification, claims, and abstract as a whole.
In various aspects, an irradiator-based power generation device is disclosed. In some aspects, the irradiator-based power generation includes a radiator layer configured to at least partially surround an irradiator, wherein the radiator layer comprises a radiator material configured to emit delta radiation in response to exposure to gamma radiation; an electrical insulation layer configured to surround the radiator layer, wherein the electrical insulation layer comprises an electrical insulation material configured to allow delta radiation to penetrate therethrough; a collector layer configured to surround the electrical insulation layer, wherein the collector layer comprises a collector material configured to collect delta radiation; a positive terminal connection electrically coupled to the irradiator, the radiator layer, or a combination thereof; and a negative terminal connection electrically coupled to the collector layer.
In various aspects, an irradiator-based power generation system is disclosed. In some aspects, the irradiator-based power generation system includes a plurality of irradiator-based power generation devices. The plurality of power generation devices can each include a device radiator layer configured to at least partially surround an irradiator, wherein the device radiator layer comprises a device radiator material configured to emit delta radiation in response to exposure to gamma radiation; a device electrical insulation layer configured to surround the device radiator layer, wherein the device electrical insulation layer comprises a device electrical insulation material configured to allow delta radiation to penetrate therethrough; a device collector layer configured to surround the device electrical insulation layer, wherein the device collector layer comprises a device collector material configured to collect delta radiation: a device positive terminal connection electrically coupled to the irradiator, the device radiator layer, or a combination thereof; and a device negative terminal connection electrically coupled to the device collector layer. The irradiator-based power generation system can further include a system positive terminal connection electrically coupled to each of the device positive terminal connections of the plurality of power generation devices and a system negative terminal connection electrically coupled to each of the device negative terminal connections of the plurality of power generation devices.
In various aspects, an irradiator-based power generation system is disclosed. In some aspects, the irradiator-based power generation system includes a system radiator layer configured to at least partially surround a plurality of irradiators, wherein the system radiator layer comprises a system radiator material configured to emit delta radiation in response to exposure to gamma radiation; a system electrical insulation layer configured to surround the system radiator layer, wherein the system electrical insulation layer comprises a system electrical insulation material configured to allow the delta radiation to penetrate therethrough; a system collector layer configured to surround the system electrical insulation layer, wherein the system collector layer comprises a system collector material configured to collect delta radiation; a system positive terminal connection electrically coupled to the system radiator layer; and a system negative terminal connection electrically coupled to the system collector layer.
These and other objects, features, and characteristics of the present disclosure, as well as the methods of operation and functions of the related elements of structure and the combination of parts and economies of manufacture, will become more apparent upon consideration of the following description and the appended claims with reference to the accompanying drawings, all of which form a part of this specification, wherein like reference numerals designate corresponding parts in the various figures. It is to be expressly understood, however, that the drawings are for the purpose of illustration and description only and are not intended as a definition of the limits of any of the aspects disclosed herein.
The various aspects described herein, together with objects and advantages thereof, may best be understood by reference to the following description, taken in conjunction with the accompanying drawings as follows.
Corresponding reference characters indicate corresponding parts throughout the several views. The exemplifications set out herein illustrate various aspects of the present disclosure, in one form, and such exemplifications are not to be construed as limiting the scope of any of the aspects disclosed herein.
Numerous specific details are set forth to provide a thorough understanding of the overall structure, function, manufacture, and use of the aspects as described in the disclosure and illustrated in the accompanying drawings. Well-known operations, components, and elements have not been described in detail so as not to obscure the aspects described in the specification. The reader will understand that the aspects described and illustrated herein are non-limiting examples, and thus it can be appreciated that the specific structural and functional details disclosed herein may be representative and illustrative. Variations and changes thereto may be made without departing from the scope of the claims.
In the following description, like reference characters designate like or corresponding parts throughout the several views of the drawings. Also in the following description, it is to be understood that such terms as “forward,” “rearward,” “left,” “right,” “above,” “below,” “upwardly,” “downwardly,” and the like are words of convenience and are not to be construed as limiting terms.
The radiation emitted by the fuel elements of nuclear reactors can be used to produce radioactive materials. For example, cobalt-60 (sometimes referred to herein as “Co-60”) can be produced from cobalt-59 (sometimes referred to herein as “Co-59”), a non-radioactive isotope of cobalt, by exposing cobalt-59 to the radiation inside the core of a nuclear reactor. Cobalt-60 has various uses in the nuclear power industry and in other industries as well.
In the context of the nuclear power industry, cobalt-60 can be created from cobalt-59 and used to generate electoral power that may be utilized to power various operations of a nuclear reactor. For example,
In other aspects, the operating principle described above with respect to
Cobalt-60 may be produced by nuclear power plants for various uses outside of the nuclear power industry. For example, cobalt-60 can be used to sterilize medical equipment, to irradiate food for perseveration and sanitation purposes, and for many other purposes. Other gamma radiation-emitting isotopes such as caesium-137 (sometimes referred to herein as “Cs-137”) may similarly be produced by nuclear power plants and used as an irradiator. Thus, the term “irradiator,” as used herein, can mean any object that includes a material having radioactive isotopes emitting gamma radiation.
Because cobalt-60 and other irradiators have many uses outside of the nuclear industry, these materials may be produced by nuclear power plants for commercial purposes. These irradiators can have a radioactivity in a range of thousands of curies (Ci) when initially produced. However, the radioactivity of these irradiators decays over time (e.g., to an activity in a range of hundreds of Ci) and eventually the depleted irradiators lose their utility in some applications. As used herein, the term “depleted irradiator” can mean any irradiator that has decreased in radioactivity compared to its initial production. In some aspects, a depleted irradiator can have a radioactivity of less than 15,000 Curies, less than 4,000 Curies, less than 3,000 Curies, less than 2,000 Curies, less than 1,500 Curies, less than 1,000 Curies, less than 500 Curies, between 500 and 15,000 Curies, between 500 and 3,000 Curies, between 500 and 2,500 Curies, between 500 and 2,000 Curies, between 500 and 1,500 Curies, between 500 and 1,000 Curies, between 50 and 2,000 Curies, between 50 and 1000 Curies, about 500 Curies, about 1,000 Curies, about 1500 Curies, about 2000 Curies, about 2500 Curies, and/or between 500 and 3000 Curies.
Current regulations require depleted irradiators to be properly disposed of or stored, which can result in an extreme financial burden to irradiator producers, such as nuclear power facilities. In some cases, this cost may ultimately outweigh the commercial benefits of producing cobalt-60 and other irradiators. Thus, there is a need for devices, systems, and methods of using irradiators after they have become depleted with respect to their initial purpose. The present disclosure provides devices, systems, and methods for generating power using gamma ray sources, such as, for example, irradiators and depleted irradiators (e.g., depleted cobalt-60 irradiators).
The power generation device 200 includes a radiator layer 202, an electrical insulation layer 204, and a collector layer 206. The irradiator 300 may be slidably inserted 207 or otherwise is positioned within the radiator layer 202. The radiator layer 202 may include a radiator layer material. In one aspect, the radiator layer material can be a high-Z material (material having a high atomic number, such as, for example, an atomic number greater than 30, such as, for example, greater than 40, greater than 50, greater than 60, or greater than 70). In another aspect, the radiator layer material can be tungsten, another high-Z material, or a combination thereof. In some aspects, the radiator layer 202 is relatively thin compared the collector layer 206. Gamma radiation emitted by the irradiator 300 can interact with the radiator layer 202 to emit delta radiation (i.e., high energy electrons). The delta radiation may be generated based on Compton and photo-electric scatting principles similar to those employed by the power supply element described above with respect to
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The collector layer 206 may be in contact with and/or surround the electrical insulation layer 204. The collector layer 206 may be configured as an outer sheath that includes a material configured to collect the delta radiation that passes through the electrical insulation layer 204, such as a metallic material configured to collect the delta radiation. The delta radiation collected by the collector layer 206 causes a voltage difference between irradiator 300 and the collector layer 206.
The power generation device 200 can include a closure lid 203 that may be threaded, welded, or otherwise attached 209 to the collector layer 206. The closure lid 203 can include a material similar to that of the collector layer 206 and can be in electrical contact with the collector layer 206. The closure lid 203 includes a positive terminal connection 210 passing therethrough. The positive terminal connection 208 is in electrical contact with the irradiator 300 and insulated 204 from the closure lid 208. The power generation device can also include a negative terminal connection 212 in electrical contact with the collector layer 206. Thus, the voltage difference between the collector layer 206 and the irradiator 300 can be used to generate an electrical current determined by a load resistance 214. Thus, the power generation device 200 may be used to generate electrical power using the irradiator 300.
The delta radiation collected by the collector layer 206 may also generate heat at the collector layer 206. This heat may be harvested using a thermal harvesting connection 216. The harvested heat energy may be used to generate power using thermo-electric conversion methods.
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The delta radiation collected by the collector layer 404 may also generate heat at the collector layer 404. This heat may be harvested using a thermal harvesting connection 414 and be used to generate power using thermo-electric conversion methods.
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The delta radiation collected by the collector layer 504 may also generate heat at the collector layer 504. This heat may be harvested using a thermal harvesting connection 514 and be used to generate power using thermo-electric conversion methods.
Exemplary power production capabilities of various power generation devices and systems described herein are provided in the examples below:
The typical range of the radioactivity of depleted cobalt-60 irradiators is between 500-2000 Curies (Ci). For the convenience of the calculation, it was assumed that the source activity is about 1000 Ci. Data provided by Mirion IST indicates that the cobalt-60 gamma sensitivity of a Tungsten self-powered detector (SPD) is equal to or more than 9×10−18 A/(R/hr)/mm2. For the convenience of this calculation, it was assumed that the sensitivity of the Tungsten layer (SPD) is about 9×1018 A/(R/hr)/mm2. In order to calculate the current that will be generated by a device similar to the power generation device 200 described above, the gamma (γ) dose rate (R/hr) associated with the source of the cobalt-60 irradiator is needed. The radiation shielding calculation tool RadPro was used calculate the dose rate of the cobalt-60 gamma (γ) corresponding to 1000 Ci activity an assumed distance of 1 mm and distance: 1000 Ci of Co-60 @0.1 cm→Dose Rate (R)=1.3×1011R/hr
The calculation also requires the surface area of the Tungsten layer (an exemplary radiator layer 202) surrounding the cobalt-60 irradiator to calculate the total current. It was assumed the surface area of the Tungsten layer surrounding the Co-60 source is the same as the surface area of the irradiator over the length containing the Co-60 pellets. The surface area of the Tungsten layer surrounding the Co-60 source is calculated as: A=π·D·L=π·(9.65)·(406)=12308.4 mm2
Using the sensitivity information for a Tungsten SPD, the expected electron current (ly) can be calculated using the relationship: ly=(9×1018) (1.3×1011) (123084)=0.0144 A/device [1000 Ci].
If R is adjusted to operate at 125 V, the corresponding power (P) is calculated as: P=V·I=(125) (0.0144)=1.8 W.
Therefore, if the individual power generation devices are combined to form the power generation system as shown in
For the power generation system shown in
If the box in the dimensions of 25″×25″×12″ is used, the effective area of the box in this example is 1.593×106 mm2 (sides+top+bottom).
The value of electron current (Iy) can be calculated using the following equation: ly=(9×10−18) (1.3×1011) (1.593×106)=1.86 A
If the R is adjusted to be operated at 125 V, the corresponding power (P) is calculated as: P=V·I=(125) (1,86)=232.5 W
In summary, the encapsulated design according to Examples 1 and 2 could produce 1 KW from a 25″×25″×12″ structure. For using an exemplary structure box design that includes the gamma harvesting design (similar to that of the power generation system of
An alternate approach would be to place cobalt-60 irradiators into a tube of high-Z metallic material, such as Tungsten, and then place the tube containing the irradiator into power generation device similar to the power generation device 200 of
Various aspects of the power generation devices and systems described herein are set out in the following clauses.
Clause 1: An irradiator-based power generation device comprising: a radiator layer configured to at least partially surround an irradiator, wherein the radiator layer comprises a radiator material configured to emit delta radiation in response to exposure to gamma radiation; an electrical insulation layer configured to surround the radiator layer, wherein the electrical insulation layer comprises an electrical insulation material configured to allow delta radiation to penetrate therethrough; a collector layer configured to surround the electrical insulation layer, wherein the collector layer comprises a collector material configured to collect delta radiation; a positive terminal connection electrically coupled to the irradiator, the radiator layer, or a combination thereof; and a negative terminal connection electrically coupled to the collector layer.
Clause 2: The power generation device of Clause 1 further comprising the irradiator.
Clause 3: The power generation device of any of Clauses 1-2, wherein the irradiator comprises a depleted irradiator.
Clause 4: The power generation device of any of Clauses 1-3, wherein the irradiator comprises cobalt-60, caesium-137, or a combination thereof.
Clause 5: The power generation device of any of Clauses 1-4, wherein the radiator material comprises tungsten.
Clause 6: The power generation device of any of Clauses 1-5, wherein the electrical insulation material comprises magnesium-oxide.
Clause 7: The power generation device of any of Clauses 1-6, further comprising a thermal harvesting connection.
Clause 8: An irradiator-based power generation system comprising: a plurality of irradiator-based power generation devices, wherein each of the plurality of power generation devices comprise: a device radiator layer configured to at least partially surround an irradiator, wherein the device radiator layer comprises a device radiator material configured to emit delta radiation in response to exposure to gamma radiation; a device electrical insulation layer configured to surround the device radiator layer, wherein the device electrical insulation layer comprises a device electrical insulation material configured to allow delta radiation to penetrate therethrough; a device collector layer configured to surround the device electrical insulation layer, wherein the device collector layer comprises a device collector material configured to collect delta radiation; a device positive terminal connection electrically coupled to the irradiator, the device radiator layer, or a combination thereof; and a device negative terminal connection electrically coupled to the device collector layer; a system positive terminal connection electrically coupled to each of the device positive terminal connections of the plurality of power generation devices; and a system negative terminal connection electrically coupled to each of the device negative terminal connections of the plurality of power generation devices.
Clause 9: The power generation system Clause 8, further comprising: a system radiator layer configured to at least partially surround the plurality of irradiator-based power generation devices, wherein the system radiator layer comprises a system radiator material configured to emit delta radiation in response to exposure to gamma radiation; a system electrical insulation layer configured to surround the system radiator layer, wherein the system electrical insulation layer comprises a system electrical insulation material configured to allow the delta radiation to penetrate therethrough; a system collector layer configured to surround the system electrical insulation layer, wherein the system collector layer comprises a system collector material configured to collect delta radiation, and wherein the system collector layer is electrically coupled to the system negative terminal connection.
Clause 10: The power generation system of any of Clauses 8-9, wherein the system radiator material comprises tungsten.
Clause 11: The power generation system of any of Clauses 8-10, wherein the system electrical insulation material comprises magnesium-oxide.
Clause 12: The power generation system of any of Clauses 8-11, further comprising a system thermal harvesting connection.
Clause 13: The power generation system of any of Clauses 8-12, wherein each of the plurality of power generation devices comprise the irradiator.
Clause 14: The power generation system of any of Clauses 8-13, wherein the irradiator comprises a depleted irradiator.
Clause 15: The power generation system of any of Clauses 8-14, wherein the irradiator comprises cobalt-60, caesium-137, or a combination thereof.
Clause 16: An irradiator-based power generation system comprising: a system radiator layer configured to at least partially surround a plurality of irradiators, wherein the system radiator layer comprises a system radiator material configured to emit delta radiation in response to exposure to gamma radiation; a system electrical insulation layer configured to surround the system radiator layer, wherein the system electrical insulation layer comprises a system electrical insulation material configured to allow the delta radiation to penetrate therethrough; a system collector layer configured to surround the system electrical insulation layer, wherein the system collector layer comprises a system collector material configured to collect delta radiation; a system positive terminal connection electrically coupled to the system radiator layer; and a system negative terminal connection electrically coupled to the system collector layer.
Clause 17: The power generation system of Clause 16, wherein the system radiator material comprises tungsten.
Clause 18: The power generation system of any of Clauses 16-17, wherein the system electrical insulation material comprises magnesium-oxide.
Clause 19: The power generation system of any of Clauses 16-18, further comprising a system thermal harvesting connection.
Clause 20: The power generation system of any of Clauses 16-19, further comprising the plurality of irradiators.
Those skilled in the art will recognize that, in general, terms used herein, and especially in the appended claims (e.g., bodies of the appended claims) are generally intended as “open” terms (e.g., the term “including” should be interpreted as “including but not limited to,” the term “having” should be interpreted as “having at least,” the term “includes” should be interpreted as “includes but is not limited to,” etc.). It will be further understood by those within the art that if a specific number of an introduced claim recitation is intended, such an intent will be explicitly recited in the claim, and in the absence of such recitation no such intent is present. For example, as an aid to understanding, the following appended claims may contain usage of the introductory phrases “at least one” and “one or more” to introduce claim recitations. However, the use of such phrases should not be construed to imply that the introduction of a claim recitation by the indefinite articles “a” or “an” limits any particular claim containing such introduced claim recitation to claims containing only one such recitation, even when the same claim includes the introductory phrases “one or more” or “at least one” and indefinite articles such as “a” or “an” (e.g., “a” and/or “an” should typically be interpreted to mean “at least one” or “one or more”): the same holds true for the use of definite articles used to introduce claim recitations.
In addition, even if a specific number of an introduced claim recitation is explicitly recited, those skilled in the art will recognize that such recitation should typically be interpreted to mean at least the recited number (e.g., the bare recitation of “two recitations,” without other modifiers, typically means at least two recitations, or two or more recitations). Furthermore, in those instances where a convention analogous to “at least one of A, B, and C, etc.” is used, in general such a construction is intended in the sense one having skill in the art would understand the convention (e.g., “a system having at least one of A, B, and C” would include but not be limited to systems that have A alone, B alone, C alone, A and B together, A and C together, B and C together, and/or A, B, and C together, etc.). In those instances where a convention analogous to “at least one of A, B, or C, etc.” is used, in general such a construction is intended in the sense one having skill in the art would understand the convention (e.g., “a system having at least one of A, B, or C” would include but not be limited to systems that have A alone, B alone, C alone, A and B together, A and C together, B and C together, and/or A, B, and C together, etc.). It will be further understood by those within the art that typically a disjunctive word and/or phrase presenting two or more alternative terms, whether in the description, claims, or drawings, should be understood to contemplate the possibilities of including one of the terms, either of the terms, or both terms unless context dictates otherwise. For example, the phrase “A or B” will be typically understood to include the possibilities of “A” or “B” or “A and B.”
It is worthy to note that any reference to “one aspect,” “an aspect,” “an exemplification,” “one exemplification,” and the like means that a particular feature, structure, or characteristic described in connection with the aspect is included in at least one aspect. Thus, appearances of the phrases “in one aspect,” “in an aspect,” “in an exemplification,” and “in one exemplification” in various places throughout the specification are not necessarily all referring to the same aspect. Furthermore, the particular features, structures or characteristics may be combined in any suitable manner in one or more aspects.
Any patent application, patent, non-patent publication, or other disclosure material referred to in this specification and/or listed in any Application Data Sheet is incorporated by reference herein, to the extent that the incorporated materials is not inconsistent herewith. As such, and to the extent necessary, the disclosure as explicitly set forth herein supersedes any conflicting material incorporated herein by reference. Any material, or portion thereof, that is said to be incorporated by reference herein, but which conflicts with existing definitions, statements, or other disclosure material set forth herein will only be incorporated to the extent that no conflict arises between that incorporated material and the existing disclosure material.
The terms “comprise” (and any form of comprise, such as “comprises” and “comprising”), “have” (and any form of have, such as “has” and “having”), “include” (and any form of include, such as “includes” and “including”) and “contain” (and any form of contain, such as “contains” and “containing”) are open-ended linking verbs. As a result, a system that “comprises,” “has,” “includes” or “contains” one or more elements possesses those one or more elements, but is not limited to possessing only those one or more elements. Likewise, an element of a system, device, or apparatus that “comprises,” “has,” “includes” or “contains” one or more features possesses those one or more features, but is not limited to possessing only those one or more features.
The term “substantially”, “about”, or “approximately” as used in the present disclosure, unless otherwise specified, means an acceptable error for a particular value as determined by one of ordinary skill in the art, which depends in part on how the value is measured or determined. In certain embodiments, the term “substantially” “about”, or “approximately” means within 1, 2, 3, or 4 standard deviations. In certain embodiments, the term “substantially”, “about”, or “approximately” means within 50%, 20%, 15%, 10%, 9%, 8%, 7%, 6%, 5%, 4%, 3%, 2%, 1%, 0.5%, or 0.05% of a given value or range.
In summary, numerous benefits have been described which result from employing the concepts described herein. The foregoing description of the one or more forms has been presented for purposes of illustration and description. It is not intended to be exhaustive or limiting to the precise form disclosed. Modifications or variations are possible in light of the above teachings. The one or more forms were chosen and described in order to illustrate principles and practical application to thereby enable one of ordinary skill in the art to utilize the various forms and with various modifications as are suited to the particular use contemplated. It is intended that the claims submitted herewith define the overall scope.
This application claims the benefit of and priority under 35 U.S.C. § 119(e) to U.S. Provisional Application No. 63/153,628, titled ELECTRIC POWER SUPPLY DEVICE CONSTRUCTED USING DEPLETED CO-60 SOURCES AND METHOD OF MANUFACTURING AND USING SAME, filed Feb. 25, 2021, the disclosure of which is hereby incorporated by reference in its entirety.
Filing Document | Filing Date | Country | Kind |
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PCT/US2022/070784 | 2/23/2022 | WO |
Number | Date | Country | |
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63153628 | Feb 2021 | US |