The project leading to this application has received funding from the European Union's Horizon 2020 research and innovation programme under grant agreement No. 828972 (nanoBRIGHT).
The present invention relates to a method and apparatus for controlling the coupling state between guided modes and plasmonic resonances in a plasmonic multimode optical fiber, said plasmonic multimode optical fiber comprising an input facet, an output facet and a plasmonic structure formed on the output facet.
The ability to realize plasmonic structures on the output facet of multimode optical fibers has enabled a set of integrated functionalities, using guided light to exploit the intrinsic properties of either Surface Plasmon Resonances (SPR) or Localized SPR (LSPR). Enhanced sensing, near-field optical microscopy, high-efficiency second-harmonic generation, plasmonic lab-on-fiber, and integrated phase shift/beam steering are primary examples of those promising applications. Still, the pivotal point of achieving full control over the photonic properties of the entire optical system in both static dynamic fashions remains unsolved.
Micro- and nano-fabrication and electromagnetic engineering indeed cannot account for the intrinsic complexity of the fiber transmission. In fact, the fiber is a highly turbid medium that substantially alters the propagation of light wavefronts up to the point that any initial spatial coherence is practically lost. Although using single mode fibers allows circumventing this problem, this comes at the cost of a limited control on the resonant patterns at the output facet, which are almost completely determined by the structural morphology. Instead, harnessing the interaction between plasmonic modes on the fiber tip and the full set of modes guided in a multimode fiber (MMF) can bring this technology to achieve its full potential.
EP2756349A2 discloses a holographic interferometric method for controlling light transmission through a multimode optical fiber in which, however, no plasmonic structure is taken in account. Plasmonic structures insert an additional layer of complexity to light propagation, making conduction electrons interacting with the light field and defining a dispersion diagram that features resonances. In addition, the plasmonic structure features sub-wavelength features, in all spatial dimensions, that play a crucial role in its response. Therefore, optical propagation rules through a generic medium (either scattering, turbid, homogeneous or not, absorbing or transparent) are insufficient to describe the physics of the coupled system composed by guided modes and plasmonic resonances.
Ditlbacher et al. “Coupling dielectric waveguide modes to surface plasmon polaritons”, Optics Express, vol. 16 No. 14, p. 10455, 7 Jul. 2008 describes the study of thin film multilayers used for the coupling of dielectric waveguide modes to surface plasmons. The combination of dielectric waveguide modes for long-range light field propagation and SPP elements enabling highly confined local light field manipulation. This paper introduces a hybrid waveguide system built from a metal-clad dielectric waveguide and a metal interface and analyzes its properties in terms of an extended layer system.
Čižmár et al. “Shaping the light transmission through a multimode optical fiber: complex transformation analysis and applications in biophotonics”. Optics Express, vol. 19 No. 20, p. 18871, 26 Sep. 2011 discloses laser light propagation through multimode optical fibers and light control at the fiber output. Beam-shaping with a spatial light modulator obtains a decomposition of the initial laser field into a series of orthogonal modes each corresponding to a different square region (sub-domain) of the SLM. A “reference mode” and a “test mode” propagating on optical fibers, interfere with output fiber facet, and the result signals of amplitude are observed in CCD camera. Subsequently, the amplitude evolution is recorded varying the phase of “test mode”. Repeating this procedure for all the input modes and then turning them ‘on’ simultaneously with the optimal phase results in optimum focusing of the signal.
Kwak et al. “Fiber-optic plasmonic probe with nanogap-rich Au nanoislands for onsite surface-enhanced Raman spectroscopy using repeated solidstate dewetting”. Journal of Biomedical Optics 24 (3), 037001, 14 Mar. 2019 describes a system made by a fiber-optic plasmonic probe for on-site SERS analysis. In particular, a multimode fiber with plasmonic nanoislands on top surface, molded with a solid-state dewetting technique. The system consists in an excitation laser coupled through the end of the multimode fiber with small biomolecules attached near the SERS-active fiber-top surface. The same fiber collects the signals, and then comes back to a spectrometer for the analysis.
L. Collard et al. “Wavefront engineering for controlled structuring of far-field intensity and phase patterns from multimodal optical fibers”, APL Photonics 6, 051301, 4 May 2021 discloses an adaptive optic method used to perform complex far-field structuring of the emission of a MMF, based on a phase modulation using a spatial light modulator at the input of a multimode fiber to generate multiple, low divergence rays with controlled angles and phase at the fiber output.
An aim of the invention is to provide a method and related apparatus allowing a dynamic and selective control of the coupling between multimodal optical fiber guided modes and the resonances of plasmonic structures realized on the output facet of a plasmonic multimode optical fiber.
In accordance with this aim, the invention proposes a method for dynamically controlling the coupling state between guided modes and plasmonic resonances in a plasmonic multimode optical fiber, said plasmonic multimode optical fiber comprising an input facet, an output facet and a plasmonic structure formed on the output facet, wherein the method comprises the steps of:
In the present disclosure, the “intensity distribution of the electromagnetic field on the plasmonic output facet” is intended as the spatial and temporal distribution of intensity of the radiative electromagnetic field as modulated by the plasmonic structures at a distance measurable within a few units of the excitation wavelength of the laser beam. In particular, such a distance may be less than 5 units of the excitation wavelength.
The “angular radiative pattern after the output facet of the plasmonic multimode optical fiber” is intended as the spatial and temporal distribution of intensity of the radiative electromagnetic field as modulated by the plasmonic structures at a distance that is significantly larger than the excitation wavelength. In particular, such a distance may be greater than 5 and up to 104 units of the excitation wavelength.
A further object of the invention is an apparatus for dynamically controlling the coupling state between guided modes and plasmonic resonances in a plasmonic multimode optical fiber, said plasmonic multimode optical fiber comprising an input facet, an output facet and a plasmonic structure formed on the output facet, wherein the apparatus comprises:
The proposed method and apparatus allow to control the coupling state between guided modes and the resonance state of plasmonic structures realized on the distal facet of a multimode optical fiber. The phase of the input wavefront into the plasmonic fiber is controlled with a wavefront shaping element (e.g. a spatial light modulator or a digital micromirror device). The resonances resulting from the interaction between conduction electrons and guided modes are monitored simultaneously in both the intensity distribution of the electromagnetic field on the output facet of the plasmonic multimode optical fiber and the radiative angular response of the plasmonic multimode optical fiber after the output facet. By defining a target optical response in one or both planes the optical system is forced to work in a well-defined coupling state, enabling:
This directly leads to applications in:
Advantageously, the plasmonic fiber can feature any type of plasmonic structure on its output facet, since the modulation input field is defined upon a measure of the available photonic states.
Further characteristics and advantages of the proposed device will be presented in the following detailed description, which refers to the attached drawings, provided purely by way of non-limiting example, in which:
The optical apparatus of
This directly leads to applications in spatially-resolved plasmonic endoscopy by exploiting Surface Enhanced Raman Scattering for molecular sensing and Extraordinary Optical Transmission.
The system shown in
The excitation block 20 is configured to send phase-modulated light (or intensity- and phase-modulated light) to the plasmonic fiber 10. A laser beam is expanded to overfill the screen of a phase-modulation element 21 (a spatial light modulator (SLM) or a digital micromirror device (DMD)), optically conjugated with the back aperture of a microscope objective (MO1) 22, focusing the modulated wavefront on the input facet 11 of the plasmonic fiber 10. The laser beam can be either continuous wave or pulsed (either fs, ps or ns), with a fixed wavelength or with a tunable wavelength in both the visible and/or the near-infrared spectral range.
The monitoring block 30 images the plasmonic output facet and its angular radiative response on two different spatially resolved detectors 31, 32 (such as CCD or CMOS cameras).
The collection block 40 collects back-propagating photons into the plasmonic fiber 10, and is employed in applications where light is recollected by the plasmonic structures 15 on the output facet 12. A spectrometer fiber is designated with 41 in
The operation method of the apparatus essentially comprises three different steps: (A) A plasmonic modes measurement step, (B) a computational step and (C) a modulation step.
Plasmonic modes excited on the output end of the plasmonic multimode optical fiber 10 are measured when applying a set of phase-modulated input light fields on the proximal end of the fiber ϕinterferej
The phase modulation in the excitation block 20 is set to a phase pattern denoted ϕinterferej
in the range [0, 2π] for a total of P=4 phase steps.
In this way, the propagation of Bscanj
The computational step aims at defining the phase modulation Φ(uin,vin) to impress at the input light field to produce a specific intensity pattern (target intensity pattern) on (xout,yout) and (uout,vout) (see
Firstly, the images FFj
Φ(uin,vin) is then applied to the phase-modulation device 21 in the excitation block 20, modulating the phase of the laser beam entering the input facet. This generates the desired patterns in the (xout,yout) or (uout,vout) and therefore sets the plasmonic fiber 10 to operate in a specific condition. The wavelength of the laser beam is chosen on the basis of the resonant wavelengths of the plasmonic structure to be targeted, in agreement with the wavelengths employed in step (A). Some possible applications are for example shown in
In a further embodiment (not shown), the output facet 12 of the plasmonic multimode optical fiber 10 further comprises nanometric optical sources deposited on the plasmonic structure 15. These nanometric optical sources may be, e.g., quantum dots or single layers of molecules. These nanometric optical sources are supplementary structures added to the plasmonic structure and have the function of producing a signal that directly measures the response in terms of non-radiative electromagnetic field.
In this embodiment, in the measurement step (A) a further set of phase modulation components can be determined in connection with the non-radiative electromagnetic field on the output facet 12 of the plasmonic multimode optical fiber 10 within a distance smaller than the excitation wavelength of the laser beam. A third detector in addition to the detectors 31 and 32 is provided to measure the light intensity patterns associated with the plasmonic modes excited by the further set of phase modulation components.
In this way, the coupling of the guided modes in the plasmonic multimode fiber with the spatial and temporal intensity distribution of the non-radiative electromagnetic field on the plasmonic output facet is measured and modulated within a distance smaller than the excitation wavelength by imaging the intensity of emission of the optical sources with nanometric dimensions.
Number | Date | Country | Kind |
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102022000003587 | Feb 2022 | IT | national |
Filing Document | Filing Date | Country | Kind |
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PCT/EP2023/054721 | 2/24/2023 | WO |