A surface-acoustic-wave (SAW) resonator uses a cavity to confine acoustic modes along the surface of an elastic substrate. SAW resonators have long been an important component in the telecommunications industry, with applications including filters and delay lines, among others. More recently, low-temperature applications of SAW devices and resonators have gained interest in the field of quantum computing, where applications include isolating superconducting qubits from unwanted interference and implementing long-lived quantum memories. Additionally, in the field of quantum acoustics, acoustic devices can be integrated with superconducting qubits to implement quantum control over mechanical degrees of freedom. Acoustic systems offer quantum technologies a favorable combination of long on-chip delays, competitive coherence times, and the ability to connect disparate quantum systems.
The present embodiments include surface-acoustic-wave (SAW) devices that reduce diffraction loss for operation at cryogenic temperatures (e.g., less than 10 K). These embodiments achieve this benefit by fabricating the device on a substrate such that SAWs propagate along a particular crystalline orientation of the substrate. This orientation is also referred to herein as a minimally-diffracting (MD) orientation. Some of the present embodiments include a SAW resonator in which a pair of acoustic reflectors (e.g., Bragg mirrors) face each other to create an acoustic cavity. The longitudinal axis of the acoustic cavity coincides with the MD orientation of the substrate at cryogenic temperatures. In other embodiments, a SAW filter or delay line is fabricated such that SAWs propagate parallel to the MD orientation.
Acoustic systems are a promising resource which offer quantum technologies a favorable combination of compact footprints, excellent coherence times, and the ability to connect disparate quantum systems [1-9]. The emergent field of circuit quantum acoustodynamics (cQAD) has leveraged these advantages to create hybrid platforms which are capable of exploring fundamental quantum physics and offer the potential for quantum computation with acoustic processors [10-17]. In particular, cQAD experiments utilizing surface acoustic wave (SAW) resonators have demonstrated increasingly sophisticated quantum control over phonons, including phonon number counting, phonon-mediated qubit-qubit entanglement, and multipartite phonon entanglement [12, 18, 19].
In a broad array of hybrid acoustic systems, maximizing coupling between a qubit and mechanical degrees of freedom is achieved by tightly confining mechanical strain [6, 9, 11, 20-22]. It can be difficult, however, to confine the strain without significantly increasing mechanical dissipation rates. In the particular example of cQAD with SAW resonators, this increase in dissipation results mainly from surface wave diffraction [12]. Consider a SAW resonator which is coupled to a nonlinear circuit element via the piezoelectric interaction of an interdigitated transducer (IDT). In such a configuration (see
Although it is possible to mitigate the deleterious effects of acoustic diffraction by appropriately curving the cavity boundaries, accomplishing this with piezoelectric media is complicated by their inherent anisotropy [3, 23, 24]; anisotropy of phase velocity, electromechanical coupling, and reflectivity must all be considered. Rather than compensating for this anisotropy, it is possible to instead exploit it into naturally suppressing acoustic diffraction. At special orientations of some piezoelectric materials (see
The present embodiments utilize MD orientations of piezoelectric crystals that are suitable for cQAD platforms. For experimental demonstrations, we chose quartz for the piezoelectric crystal due its extremely low bulk mechanical losses at millikelvin temperatures and its relatively strong piezoelectricity [25]. An MD orientation of quartz for room-temperature SAW devices was previously identified [26, 27]. However, the temperature dependence of the piezoelectric and elastic coefficients of quartz causes this cut to lose its MD property as it is cooled to ultra-low temperatures. This motivates the search for an orientation of quartz which minimizes SAW diffraction in the low-temperature limit.
We used finite element method (FEM) simulations to model diffraction and beam-steering for ultra-low temperature quartz to identify an MD orientation suitable for quantum experiments. From these simulations, we identify an orientation of quartz at Euler angles (ψ, ϕ, θ)=(0°, 40.2°, 23.4°) [28]. This orientation minimizes SAW diffraction and beam-steering to second-order when cooled to ultra-low temperatures. Experimentally, we fabricated SAW resonators with two flat acoustic reflectors (see
Minimal diffraction in anisotropic materials can be understood as an effect of beam-steering, a phenomenon that causes a beam in an anisotropic medium to propagate in a direction which is not normal to the wavefront. As shown in
Beam-steering vanishes at angle θ0 for which v(θ) exhibits a stationary point. However, any finite-width IDT oriented at θ0 will transduce SAWs at a spectrum of angles around θ0 which, on an anisotropic substrate, necessarily exhibit beam-steering. The second-order diffractive spread of the beam width due to this off-axis beam-steering is characterized by the diffraction parameter γ,
which can be used to calculate the diffraction-limited quality factor Qd of a flat SAW cavity on an anisotropic substrate [29],
Diffraction is reduced (compared to isotropic substrates) for materials where −2<γ<0 and otherwise increased. ST quartz, for example, exhibits accelerated wave diffraction γ=0.378 and isotropic materials exhibit γ=0. Minimal diffraction occurs when γ=−1, a special condition such that beam-steering at small angles δ around some orientation θ0 follows η(S) ≈−δ. In this circumstance, waves transduced at angle θ0+δ by a finite-width IDT will propagate in the direction θ0. Thus when γ=−1, as shown in
We thus search for an orientation of quartz which (i) exhibits η≈0°, (ii) exhibits γ≈−1, (iii) and is tolerant to potential errors in manufacturer cutting. Due to the trigonal structure of α-quartz, three Euler angles (ψ, ϕ, θ) are necessary to uniquely describe the orientation of a device relative to some crystallographic axes [28]. In the following discussion, we consider only cuts where p=0°, i.e., singly-rotated cuts. Singly-rotated cuts are easier to cut than doubly-rotated cuts, even though the present embodiments may still work with double-rotated cuts. The remaining angles (0, 0) are illustrated in
Using FEM simulations, we generated velocity curves v(ϕ, θ) in the space (ψ, ϕ, θ)=(0°, −90°: 90°, 0°: 180°) and applied Eqns. 1 and 2 to calculate η and γ [30]. The basis of the simulations was a 3D unit cell with two pairs of periodic mechanical and electric boundary conditions in the longitudinal and transverse dimensions. An eigenfrequency study revealed surface wave modes for a particular orientation, and the velocity of the lowest frequency mode was traced to produce v(0, 0). From the simulation we also determined the SAW polarization supported by a given orientation. In particular, we searched for Rayleigh-(R) polarized SAWs, which exhibit less propagation attenuation than shear-horizontal (SH) or other non-Rayleigh polarizations [1]. The crystallographic orientation was specified by rotating the piezoelectric and elastic tensors relative to the unit cell axes. To model low temperature quartz, we used piezoelectric and elastic coefficients for right-handed α-quartz measured at 5 K [31]. Simulated velocity curves for MD (ϕ=40.2°) and ST (ϕ=−47.25°) quartz are shown in
We procured COLD quartz wafers from a vendor with quoted tolerance (±0.1°, ±0.03°, ±0.1°). To test the performance of the substrate, we first fabricated a series of one-port resonators and varied the angle θ at which each device is oriented relative to the crystallographic axes. Double-finger IDTs were patterned from a 25 nm aluminum film, and SAWs were confined by etched Bragg mirror gratings with 250 elements and a reflectivity of 1-2% per element [1, 29]. The resonators were designed with wavelength λ=7.28 μm and a mirror-to-mirror cavity length of 150λ. These resonators were designed with a narrow aperture (W˜10λ) so that losses are dominated by diffraction.
In
To measure γ, we fabricated a series of SAW resonators at θ=23.4° with aperture widths W ranging from 5λ to 40λ. In
There are two approaches to reducing these residual beam-steering losses: compensate for ηeff with device geometry or choose an orientation for which all odd-order derivatives of v(θ) vanish. Preliminary experiments suggest that it is possible to mitigate ηeff loss by fabricating resonators which have a mirror aperture slightly wider than the IDT aperture W to capture the misaligned portion of the beam. Alternatively, the phenomenon of narrow-aperture-induced effective beam-steering can be eliminated entirely by choosing an orientation which lies along a crystalline symmetry axis so that the velocity profile is fully symmetric about the propagation axis. Unfortunately, of the two symmetry-axis R-polarized SAW orientations identified in Table 1, both exhibit very low k2. Doubly-rotated cuts, in which ψ≠0°, may yield MD orientations of quartz with both greater symmetry in v(θ) and nonzero k2.
Improving the lifetimes of mechanical resonators coupled to superconducting circuits is critical for maximizing the capabilities of cQAD systems. By discovering a substrate which naturally suppresses SAW diffraction losses, we have provided a solution to the dominant loss source observed in previous SAW-qubit devices [12]. This will allow this class of devices to be pushed further into the strong-dispersive regime to facilitate the exploration of multimodal quantum information processing [12, 33, 34]. COLD quartz may also be useful in the creation of low-loss cryogenic delay lines, phononic waveguides, and electro-acoustic phase modulators [35-39]. Crystallographic optimization has become less common in recent decades as standard crystal orientations for acoustic devices have emerged. In studying a non-standard orientation of quartz, we highlight the remaining utility of crystallographic engineering for quantum applications. Supplementary Material
Unit Cell Simulations
Calculating velocity for a particular crystallographic orientation is accomplished with unit cell simulations.
Electromechanical Coupling
The electromechanical coupling coefficient k2 is defined by
where vf and vs are the free and shorted velocities of a SAW propagating on a substrate [1]. The shorted velocity corresponds to a surface with an idealized metal coating that shorts the longitudinal component of the electric field; we simulated this by adding a grounding boundary condition to the top boundary. We use piezoelectric tensors corresponding to room temperature values and repeat the eigenfrequency search with 1° resolution over the parameter space.
Effective Beam-Steering
To understand the effect of velocity profile asymmetry on SAWs, we simulated far-field SAW propagation with the angular spectrum of waves technique [41]. The SAW displacement field is proportional to
where x and z are the transverse and longitudinal coordinates, W is the width of a transducer launching SAWs along the x axis from −W/2 to W/2, and kx and kz are the components of the wave vector in the x and z directions given that
k
z(kx)2=k({circumflex over (k)})2−kx, (6)
where
k({circumflex over (k)})=2πf/v({circumflex over (k)}), (7)
v({circumflex over (k)}) is the phase velocity in wave-vector direction k and f is the frequency. In
and plot this both on the figure and below as a function of z. The center of intensity shifts approximately linearly against z, corresponding to an effective beam-steering ηeff≠0.6°.
This phenomenon can be attributed to the asymmetry of the velocity profile. The ideal minimally-diffracting profile v(θ)∝cos(θ) for all θ produces an angular beam-steering profile η(θ)=−θ which facilitates uniaxial transduction of SAWs. However, it is generally sufficient to match the ideal profile for only several degrees about the maximum; wavevector contributions are most significant from these angles. Indeed, the COLD quartz velocity profile approximates a cosine well for ±2° around 23.4° before deviating. This deviation is necessarily asymmetric as COLD quartz is not oriented along a crystalline symmetry axis. In particular, the high-angle side (θ>23.4°) diverges more quickly and SAWs transduced at these angles do not exhibit large enough beam-steering to achieve an MD wavefront. Contributions from these angles will thus ‘steer’ the propagating SAW towards higher angles, and ηeff will be minimized at some higher angle. The degree to which a given wave vector-direction k contributes to the propagating field is dependent on the width of transducer; this is captured in Eqn. 5 by the sinc-term sin(kxW/2)/kx. The narrower the IDT aperture W1, the more impactful these high-angle deviations become, contributing to a higher angle at which ηeff is minimized.
For wider aperture resonators (W≥15λ), this phenomenon is largely negligible. For narrow-aperture devices, however, mitigating this added source of loss may be necessary. This can be accomplished by shifting the orientation of the transducer to the angle of minimal ηeff or by widening the mirror width compared to the IDT aperture W.
Fabrication
Photoresist patterning was performed with an ASML 5500/100D Wafer Stepper, which supports a 400 nm resolution and 90 nm alignment between lithographic layers. This allows for excellent angular precision while using optical lithography; the smallest device feature size is 910 nm. Wafer preparation began with a Nanostrip etch to remove residual organics followed by evaporation of a 25 nm aluminum film covering the entire 3-inch wafer which will later form the metallized features. Photoresist (nLOF 2020) was then spun onto the wafer, and alignment mark patterns for the wafer stepper were exposed in negative. A 10-nm layer of titanium and a 100-nm layer of gold were evaporated and the films were lifted off to leave behind the alignment marks.
Device fabrication is a simple two layer process for one-port SAW resonators. First, SPR660 photoresist was spun onto the wafer and the stepper was used to pattern regions where the aluminum film was to be etched away. This layer defined the CPW, IDT, and cavity regions. The metal was etched with Transene etchant type A. Photoresist was re-spun and Bragg mirror gratings were patterned in the cavity region. The mirror gratings were etched into the quartz with an Oxford PlasmaLab ICP-380 using fluorine. The target depth for this etch was 73 nm or h/λ=1%, which was found to yield a 1.5% reflectivity per grating element.
In embodiments, the term “cryogenic” refers to temperatures accessible via liquid-nitrogen cooling (i.e., less than 77 K). In some of these embodiments, the cryogenic temperatures are less than 10 K or 4.2 K, which are accessible via liquid-helium cooling. Temperatures as low as a few millikelvin can be achieved with helium dilution refrigerator. Accordingly, the present embodiments may be used with such dilution refrigerators or other cryogenic devices.
There are several ways to excite modes of the acoustic cavity 128. In the example of
The SAWs 122 travel in directions 124 and 125, parallel to the cavity axis 130 and along the surface 140 of the substrate 110, toward the acoustic reflectors 120 and 121. The acoustic reflectors 120 and 121 at least partially reflect the SAWs 122 to create reflected SAWs that propagate along directions 127 and 126, respectively. Reflection of SAWs 122 back-and-forth between the acoustic reflectors 120 and 121 can therefore excite one or more modes of the acoustic cavity 128, thereby transferring energy from the SAWs 122 to the cavity modes. Coupling of energy from the SAWs 122 into the cavity mode varies with the detuning between the frequency of the SAWs 122 and the resonance frequencies of the cavity modes. The frequency of the SAWs 122 can be adjusted, in part, by the interdigit spacing of the fingers of the electrodes 112 and 114.
In
In some embodiments, the acoustic cavity 128 is excited without electrical transduction. In these embodiments, the SAW resonator 900 may exclude the electrodes 112 and 114. Furthermore, the anisotropic crystal forming the substrate 110 need not be piezoelectric. In one of these embodiments, modes of the acoustic cavity 128 are excited with phonons that are transmitted through one of the acoustic reflectors 120 and 121. In another of these embodiments, a SAW may be launched into the acoustic cavity 128 at a non-zero angle relative to the cavity axis 130. In this case, diffraction or scattering may be used to couple some of the energy of the SAW into a cavity mode. Another mechanism for coupling energy into the acoustic cavity 128 may be used without departing from the scope hereof.
The substrate 110 may be formed from any anisotropic crystal known in the art. In some embodiments, the crystal is piezoelectric. As described above, quartz (e.g., α-quartz) is one such piezoelectric crystal. Other examples of piezoelectric crystals include, but are not limited to, silicon carbide (SiC), gallium arsenide (GaAs), zinc oxide (ZnO), aluminum nitride (AlN), lithium niobate (LiNbO3), and lithium tantalate (LiTaO3), and potassium niobate (KNbO3). Examples of non-piezoelectric crystals include, but are not limited to, sapphire and silicon. It should be understand that the particular values of the Euler angles (ψ, ϕ, θ) described above apply only to the MD orientation of α-quartz at cryogenic temperatures. Since the MD orientation depends on crystal properties, the values of the Euler angles (ψ, ϕ, θ) for the MD orientation will be different than those presented above when the substrate 110 is fabricated from an anisotropic crystal other than α-quartz. The substrate 110 may be cut such that the MD orientation is parallel to an edge (e.g., the length) of the substrate 110. In this case, the acoustic reflectors 120 and 121 can be fabricated such that the cavity axis 130 is parallel to the edge.
Propagation of SAWs with minimal diffraction can also be used to reduce energy loss in devices other than resonators. Accordingly, the present embodiments include other types of SAW devices that operate with MD orientations of anisotropic crystals at cryogenic temperatures. For examples, SAW filters and delay lines use input and output transducers fabricated on a piezoelectric substrate. The input and output transducers may be positioned such that the transmission direction of SAWs from the input transducer to the output transducer is aligned with an MD orientation of the piezoelectric substrate (at cryogenic temperatures). Advantageously, the input and output transducers can be constructed with narrower apertures, as compared to SAW filters that do not use an MD orientation. Alternatively, the input and output transducers can be separated by a greater distance.
Changes may be made in the above methods and systems without departing from the scope hereof. It should thus be noted that the matter contained in the above description or shown in the accompanying drawings should be interpreted as illustrative and not in a limiting sense. The following claims are intended to cover all generic and specific features described herein, as well as all statements of the scope of the present method and system, which, as a matter of language, might be said to fall therebetween.
This application claims priority to U.S. Provisional Patent Application No. 63/268,630, filed on Feb. 28, 2022, the entirety of which is incorporated herein by reference.
This invention was made with government support under grant number N00014-20-1-2833 awarded by the Office of Naval Research. The government has certain rights in the invention.
Number | Date | Country | |
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63268630 | Feb 2022 | US |