The present disclosure relates generally to a radioisotope activity surveillance apparatus, system and method. More particularly, the present disclosure relates generally to a radioisotope activity surveillance apparatus, system and method for use with fuel assembly insert targets. The present disclosure also pertains to techniques for measuring and analyzing signals received from the surveillance tool and calculating the radioisotope activity of a target assembly.
The production of desired amounts of medical or industrial radioisotopes inside a commercial power generating reactor, such as Cobalt-60 (Co-60), requires that a target material is placed inside the reactor and receive a specific neutron flux exposure level for a minimum amount of reactor operating time. In order to determine whether the irradiation target is actually ready to harvest requires that the activity level of the desired radioisotope inside the target assembly is measured. Thus, there is a need for an apparatus, system, and method to measure the activity of a desired radioisotope during a reactor refueling outage to determine whether to extract and process the irradiation target material. There is also a need to determine the progress of the production of the desired radioisotope during refueling outages that occur prior to the expected harvesting time.
In one aspect, the present disclosure provides a radioisotope activity surveillance system, comprising a fuel rod assembly comprising a plurality of nuclear fuel rods; a target assembly comprising: a top nozzle comprising an orifice plate; and at least one target material rod fixedly coupled to the orifice plate, wherein the at least one target material rod is slidably disposed within the fuel rod assembly; and a sensing assembly defining an opening sized and configured to receive the target assembly therethrough, the sensing assembly comprising a self-powered detector assembly to detect radioisotope activity of the target rod material.
In another aspect of the radioisotope activity surveillance system, the self-powered detector assembly comprises: a sensing portion comprising an emitter wire; and a signal wire electrically coupled to the emitter wire; wherein the emitter wire is made of a prompt responding gamma sensitive material and generates an electrical current when exposed to gamma radiation; and wherein the emitter wire and the signal wire are encased in an outer sheath.
In another aspect of the radioisotope activity surveillance system, the emitter wire comprises platinum.
In another aspect of the radioisotope activity surveillance system, the signal wire is made of steel.
In another aspect of the radioisotope activity surveillance system, wherein the outer sheath is made of steel. In another aspect of the radioisotope activity surveillance system, the outer sheath is filled with an electrical insulator material. In another aspect of the radioisotope activity surveillance system the electrical insulator material is Magnesium Oxide (MgO).
In another aspect of the radioisotope activity surveillance system, the sensing assembly comprises: an inner case; an outer shielding; and a space defined therebetween to accommodate a spiral wound sensing portion of the self-powered detector assembly.
In another aspect of the radioisotope activity surveillance system, the outer shielding is constructed of a material to shield the sensing portion emitter wire from gamma radiation originating from outside the sensing assembly. In another aspect of the radioisotope activity surveillance system, the outer shielding is constructed of tungsten (W).
In another aspect of the radioisotope activity surveillance system, the sensing assembly is connected to a handle. In another aspect of the radioisotope activity surveillance system, the handle is configured to position the sensing assembly at atop of the target assembly containing the target material rods to be extracted from/inserted into the fuel rod assembly.
In one aspect, the present disclosure provides a method for measuring a self-powered detector signal to calculate radioisotope activity of a target assembly, a target assembly comprising a top nozzle comprising an orifice plate and at least one target material rod fixedly coupled to the orifice plate, wherein the at least one target material rod is slidably disposed within the fuel rod assembly. The method comprises positioning a sensing assembly over a fuel rod assembly, the sensing assembly defining an opening sized and configured to receive the target assembly therethrough, the sensing assembly comprising a self-powered detector assembly to detect radioisotope activity of the target rod material; obtaining, by the sensing assembly, a first background gamma radiation signal measurement from external gamma sources; recording the first background gamma radiation signal measurement by a recorder; passing the target assembly through the sensing assembly at a constant rate; recording, by the recorder, a measured self-powered detector signal current (I) as a function of time while the target assembly passes through the sensing assembly; obtaining a second background gamma radiation signal measurement from external gamma sources after the target assembly is fully passed through the sensing assembly; and recording the second background gamma radiation signal measurement by the recorder.
In another aspect, the method comprises determining total radioisotope activity of the target assembly by integrating a fitted function of the measured self-powered detector signal current (I) versus time over an active length of the target assembly.
In another aspect, the method comprises determining an integrated region based on a withdrawal/insertion rate and the measured self-powered detector signal current (I) recorded when an active portion of the target assembly is inside the opening defined by the sensing assembly.
In another aspect of the method the first and second background gamma radiation signal measurements from external gamma sources are obtained by measuring a current (I) through the self-powered detector signal cable.
In one aspect, the present disclosure provides a method for analyzing total activity of a desired radioisotope. The method comprises recording a self-powered detector signal as function of time while a target assembly is passed at a constant rate through a sensing assembly, wherein the target assembly contains the target material rods being used to create the desired radioisotope; creating a representation of the background-corrected measured self-powered detector signal as a function of position along the target assembly; creating a function that provides a fitted representation of the measured self-powered detector signal as a function of the target assembly position (L); integrating the function over a length of the target assembly that contains the target material rods being used to create the desired radioisotope; and converting the integrated value to gamma activity based on gamma sensitivity.
In another aspect, the method comprises determining whether to harvest the desired radioisotope based on the gamma activity.
In another aspect of the method the function has the form of:
The foregoing summary is illustrative only and is not intended to be in any way limiting. In addition to the illustrative aspects, embodiments, and features described above, further aspects, embodiments, and features will become apparent by reference to the drawings and the following detailed description.
Various features of the embodiments described herein, together with advantages thereof, may be understood in accordance with the following description taken in conjunction with the accompanying drawings as follows.
Corresponding reference characters indicate corresponding parts throughout the several views. The exemplifications set out herein illustrate various embodiments of the invention, in one form, and such exemplifications are not to be construed as limiting the scope of the invention in any manner.
In one aspect, the present disclosure provides a radioisotope activity surveillance apparatus, system and method to measure the activity of a desired radioisotope during a reactor refueling outage to determine whether to extract and process the irradiation target material. In another aspect, the present disclosure provides a radioisotope activity surveillance apparatus, system and method to determine the progress of the production of the desired radioisotope during refueling outages that occur prior to the expected harvesting time.
In one aspect, the present disclosure provides an apparatus, system, and method to confirm design predictions of a production rate of a desired radioisotope and determine whether the activity of the desired radioisotope is high enough to begin harvesting operations. The apparatus has no moving parts and is not susceptible to operating characteristic changes due to radiation exposure.
In one aspect, the apparatus, system, and method according to the present disclosure enables the production of radioisotopes, such as Co-60, for example, above a certain minimum required activity level without the need to cut open the target assembly rodlets. The application of the apparatus, system, and method according to the present disclosure can reduce certain commercial risks associated with the production of radioisotopes.
Turning now to the figures,
The production of desired amounts of medical or industrial radioisotopes inside a commercial power generating reactor, such as Co-60, requires that the target material rods 108 are inserted into the fuel rod assembly 104 inside the reactor to receive a specific level of neutron flux exposure for a minimum amount of reactor operating time. In order to determine whether the irradiation target material rods 108 are ready to be harvested requires that the activity level of the desired radioisotope inside the target assembly 102 is measured. The radioisotope activity surveillance system 100 is employed to measure the activity of a desired radioisotope during a reactor refueling outage so a decision on whether to extract and process the irradiation target material rods 108 can be made. In use, the radioisotope activity surveillance system 100 allows the progress of the production of the desired radioisotope material to be determined during refueling outages that occur prior to the expected harvesting time.
The fuel rod assembly 104 comprises a plurality of fuel rods 118. Grid spacers 120 hold the fuel rod 118 bundles in position, maintain appropriate rod-to-rod clearance, and enhance critical heat flux. The target material rods 108 are slidably disposed between the fuel rods 118.
The sensing assembly 106 defines an opening 112 large enough to receive the target assembly 102. In the example illustrated in
In various aspects, the SPD assembly 200 emitter wire 204 comprises an emitter core of at least one material selected from nickel, iron, titanium and alloys based on these metals, and an emitter outer layer around the core which has a thickness in the range of the order of 0.03 mm to of the order of 0.062 mm and which is of at least one material selected from platinum, tantalum, osmium, molybdenum and cerium. With this construction, by increasing the emitter diameter beyond the optimum for a solid platinum emitter, the ratio of neutron to gamma-ray sensitivity, and hence the prompt response fraction, is increased while an acceptably small burnup rate is maintained. Larger diameter emitters of this construction have response characteristics that closely match those required for a fuel power detector in, for example, heavy-water-moderated, natural uranium power reactors. The emitter core is preferably of inconel (Trademark) and the emitter jacket is preferably of platinum.
The outer shielding 304 of the sensing assembly 106 may be constructed of a material, such as tungsten (W), that will shield the sensing portion 202 of the SPD emitter wire 204 from gamma radiation originating from outside the sensing assembly 106. The inner case 302 of the sensing assembly 106 is constructed of a material, such as steel, for example, to minimize the attenuation of the gamma radiation being used to determine the activity of the target material on the target material rods 108. The sensing assembly 106 is sealed to prevent water intrusion during use.
The sensing assembly 106 is connected to the handle 114 that serves as a means for positioning the sensing assembly 106 at the top of the target assembly 102 containing the target material rods 108 to be extracted from/inserted into the fuel rod assembly 104. The length of the handle 114 is sufficient to facilitate accessibility from the bridge in a refueling pool or casking pool. The handle 114 also serves as a conduit for the SPD signal wire 116 portion of the SPD assembly 200. The total length of the SPD signal wire 116 is sufficient to allow the SPD signal to be measured at the desired location in a target harvest area. The height ‘H’ of the sensing assembly 106 may be selected to be about 10 in. although the present disclosure should not be limited in this context.
In aspect, the activity measurement system 100 shown in
After positioning 402 the sensing assembly 106 into the desired position, a first background gamma radiation signal measurement from external gamma sources is obtained 404 by measuring a current (I) through the SPD signal cable 116, with a desired measurement accuracy, before passing (extracting/inserting) the target assembly 102 through the sensing assembly 106. The measured current (I) representative of the background gamma radiation is then recorded 406 by the recorder 124.
After recording 406 the background gamma radiation signal current (I), the target assembly 102 is passed 408 (withdrawn or inserted) through the sensing assembly 106 at a constant rate. The rate should be controlled to allow the measurement accuracy of the measured SPD signal current (I) to be controlled. The measured SPD signal current (I) as a function of time is recorded 410 by the recorder 124 while the target assembly 102 passes 408 through the sensing assembly 106. After the target assembly 102 is fully passed 408 through the sensing assembly, a second background gamma radiation signal measurement from external gamma sources is obtained 412 and the measured SPD signal current (I) is recorded 414 by the recorder 124. The method 400 is repeated as needed to measure gamma radiation signals for all the desired target assemblies 102.
The total radioisotope activity of the desired radioisotope of the target assembly 102 is determined by integrating a fitted function of the measured self-powered detector signal current (I) versus time over the active length of the target assembly 102. The integrated region is determined using the withdrawal/insertion 408 rate and measured self-powered detector signal current (I) data when the active portion of the target assembly 102 is inside the opening 112 defined by the sensing assembly 106. An example of the analysis method used in one approach is described by the process 500 described in
Various aspects of the subject matter described herein are set out in the following examples.
Example 1. A radioisotope activity surveillance system, comprising: a fuel rod assembly comprising a plurality of nuclear fuel rods; a target assembly comprising: a top nozzle comprising an orifice plate; and at least one target material rod fixedly coupled to the orifice plate, wherein the at least one target material rod is slidably disposed within the fuel rod assembly; and a sensing assembly defining an opening sized and configured to receive the target assembly therethrough, the sensing assembly comprising a self-powered detector assembly to detect radioisotope activity of the target rod material.
Example 2. The radioisotope activity surveillance system of Example 1, wherein the self-powered detector assembly comprises: a sensing portion comprising an emitter wire; and a signal wire electrically coupled to the emitter wire; wherein the emitter wire is made of a prompt responding gamma sensitive material and generates an electrical current when exposed to gamma radiation; and wherein the emitter wire and the signal wire are encased in an outer sheath.
Example 3. The radioisotope activity surveillance system of any one or more of Examples 1 through 2, wherein the emitter wire comprises platinum.
Example 4. The radioisotope activity surveillance system of any one or more of Examples 1 through 3, wherein the signal wire is made of steel.
Example 5. The radioisotope activity surveillance system of any one or more of Examples 1 through 4, wherein the outer sheath is made of steel.
Example 6. The radioisotope activity surveillance system of any one or more of Examples 1 through 5, wherein the outer sheath is filled with an electrical insulator material.
Example 7. The radioisotope activity surveillance system of any one or more of Examples 1 through 6, wherein the electrical insulator material is Magnesium Oxide (MgO).
Example 8. The radioisotope activity surveillance system of any one or more of Examples 1 through 7, wherein the sensing assembly comprises: an inner case; an outer shielding; and a space defined therebetween to accommodate a spiral wound sensing portion of the self-powered detector assembly.
Example 9. The radioisotope activity surveillance system of any one or more of Examples 1 through 8, wherein the outer shielding is constructed of a material to shield the sensing portion emitter wire from gamma radiation originating from outside the sensing assembly.
Example 10. The radioisotope activity surveillance system of any one or more of Examples 1 through 9, wherein the outer shielding is constructed of tungsten (W).
Example 11. The radioisotope activity surveillance system of any one or more of Examples 1 through 10, wherein the sensing assembly is connected to a handle.
Example 12. The radioisotope activity surveillance system of any one or more of Examples 1 through 11, wherein the handle is configured to position the sensing assembly at atop of the target assembly containing the target material rods to be extracted from/inserted into the fuel rod assembly.
Example 13. A method for measuring a self-powered detector signal to calculate radioisotope activity of a target assembly, a target assembly comprising a top nozzle comprising an orifice plate and at least one target material rod fixedly coupled to the orifice plate, wherein the at least one target material rod is slidably disposed within the fuel rod assembly, the method comprising: positioning a sensing assembly over a fuel rod assembly, the sensing assembly defining an opening sized and configured to receive the target assembly therethrough, the sensing assembly comprising a self-powered detector assembly to detect radioisotope activity of the target rod material; obtaining, by the sensing assembly, a first background gamma radiation signal measurement from external gamma sources; recording the first background gamma radiation signal measurement by a recorder; passing the target assembly through the sensing assembly at a constant rate; recording, by the recorder, a measured self-powered detector signal current (I) as a function of time while the target assembly passes through the sensing assembly; obtaining a second background gamma radiation signal measurement from external gamma sources after the target assembly is fully passed through the sensing assembly; and recording the second background gamma radiation signal measurement by the recorder.
Example 14. The method of Example 13, comprising determining total radioisotope activity of the target assembly by integrating a fitted function of the measured self-powered detector signal current (I) versus time over an active length of the target assembly.
Example 15. The method of any one or more of Examples 13 through to 14, comprising determining an integrated region based on a withdrawal/insertion rate and the measured self-powered detector signal current (I) recorded when an active portion of the target assembly is inside the opening defined by the sensing assembly.
Example 16. The method of any one or more of Examples 13 through 15, wherein the first and second background gamma radiation signal measurements from external gamma sources are obtained by measuring a current (I) through the self-powered detector signal cable.
Example 17. A method for analyzing total activity of a desired radioisotope, the method comprising: recording a self-powered detector signal as function of time while a target assembly is passed at a constant rate through a sensing assembly, wherein the target assembly contains the target material rods being used to create the desired radioisotope; creating a representation of the background-corrected measured self-powered detector signal as a function of position along the target assembly; creating a function that provides a fitted representation of the measured self-powered detector signal as a function of the target assembly position (L); integrating the function over a length of the target assembly that contains the target material rods being used to create the desired radioisotope; and converting the integrated value to gamma activity based on gamma sensitivity.
Example 18. The method of Example 17, comprising determining whether to harvest the desired radioisotope based on the gamma activity.
Example 19. The method of any one or more of Examples 17 through 18, wherein the function has the form of: −y(L)=a0+a1(L)+a2(L)2+a3(L)3+ . . . +an(L)n.
While specific embodiments of the invention have been described in detail, it will be appreciated by those skilled in the art that various modifications and alternatives to those details could be developed in light of the overall teachings of the disclosure and that selected elements of one or more of the example embodiments may be combined with one or more elements from other embodiments without varying from the scope of the disclosed concepts. Accordingly, the particular embodiments disclosed are meant to be illustrative only and not limiting as to the scope of the invention which is to be given the full breadth of the appended claims and any and all equivalents thereof.
Those skilled in the art will recognize that, in general, terms used herein, and especially in the appended claims (e.g., bodies of the appended claims) are generally intended as “open” terms (e.g., the term “including” should be interpreted as “including but not limited to,” the term “having” should be interpreted as “having at least,” the term “includes” should be interpreted as “includes but is not limited to,” etc.). It will be further understood by those within the art that if a specific number of an introduced claim recitation is intended, such an intent will be explicitly recited in the claim, and in the absence of such recitation no such intent is present. For example, as an aid to understanding, the following appended claims may contain usage of the introductory phrases “at least one” and “one or more” to introduce claim recitations. However, the use of such phrases should not be construed to imply that the introduction of a claim recitation by the indefinite articles “a” or “an” limits any particular claim containing such introduced claim recitation to claims containing only one such recitation, even when the same claim includes the introductory phrases “one or more” or “at least one” and indefinite articles such as “a” or “an” (e.g., “a” and/or “an” should typically be interpreted to mean “at least one” or “one or more”); the same holds true for the use of definite articles used to introduce claim recitations.
In addition, even if a specific number of an introduced claim recitation is explicitly recited, those skilled in the art will recognize that such recitation should typically be interpreted to mean at least the recited number (e.g., the bare recitation of “two recitations,” without other modifiers, typically means at least two recitations, or two or more recitations). Furthermore, in those instances where a convention analogous to “at least one of A, B, and C, etc.” is used, in general such a construction is intended in the sense one having skill in the art would understand the convention (e.g., “a system having at least one of A, B, and C” would include but not be limited to systems that have A alone, B alone, C alone, A and B together, A and C together, B and C together, and/or A, B, and C together, etc.). In those instances where a convention analogous to “at least one of A, B, or C, etc.” is used, in general such a construction is intended in the sense one having skill in the art would understand the convention (e.g., “a system having at least one of A, B, or C” would include but not be limited to systems that have A alone, B alone, C alone, A and B together, A and C together, B and C together, and/or A, B, and C together, etc.). It will be further understood by those within the art that typically a disjunctive word and/or phrase presenting two or more alternative terms, whether in the description, claims, or drawings, should be understood to contemplate the possibilities of including one of the terms, either of the terms, or both terms unless context dictates otherwise. For example, the phrase “A or B” will be typically understood to include the possibilities of “A” or “B” or “A and B.”
With respect to the appended claims, those skilled in the art will appreciate that recited operations therein may generally be performed in any order. Also, although various operational flow diagrams are presented in a sequence(s), it should be understood that the various operations may be performed in other orders than those which are illustrated, or may be performed concurrently. Examples of such alternate orderings may include overlapping, interleaved, interrupted, reordered, incremental, preparatory, supplemental, simultaneous, reverse, or other variant orderings, unless context dictates otherwise. Furthermore, terms like “responsive to,” “related to,” or other past-tense adjectives are generally not intended to exclude such variants, unless context dictates otherwise.
It is worthy to note that any reference to “one aspect,” “an aspect,” “an exemplification,” “one exemplification,” and the like means that a particular feature, structure, or characteristic described in connection with the aspect is included in at least one aspect. Thus, appearances of the phrases “in one aspect,” “in an aspect,” “in an exemplification,” and “in one exemplification” in various places throughout the specification are not necessarily all referring to the same aspect. Furthermore, the particular features, structures or characteristics may be combined in any suitable manner in one or more aspects.
Any patent application, patent, non-patent publication, or other disclosure material referred to in this specification and/or listed in any Application Data Sheet is incorporated by reference herein, to the extent that the incorporated materials is not inconsistent herewith. As such, and to the extent necessary, the disclosure as explicitly set forth herein supersedes any conflicting material incorporated herein by reference. Any material, or portion thereof, that is said to be incorporated by reference herein, but which conflicts with existing definitions, statements, or other disclosure material set forth herein will only be incorporated to the extent that no conflict arises between that incorporated material and the existing disclosure material.
The terms “comprise” (and any form of comprise, such as “comprises” and “comprising”), “have” (and any form of have, such as “has” and “having”), “include” (and any form of include, such as “includes” and “including”) and “contain” (and any form of contain, such as “contains” and “containing”) are open-ended linking verbs. As a result, a system that “comprises,” “has,” “includes” or “contains” one or more elements possesses those one or more elements, but is not limited to possessing only those one or more elements. Likewise, an element of a system, device, or apparatus that “comprises,” “has,” “includes” or “contains” one or more features possesses those one or more features, but is not limited to possessing only those one or more features.
In summary, numerous benefits have been described which result from employing the concepts described herein. The foregoing description of the one or more forms has been presented for purposes of illustration and description. It is not intended to be exhaustive or limiting to the precise form disclosed. Modifications or variations are possible in light of the above teachings. The one or more forms were chosen and described in order to illustrate principles and practical application to thereby enable one of ordinary skill in the art to utilize the various forms and with various modifications as are suited to the particular use contemplated. It is intended that the claims submitted herewith define the overall scope of the disclosure.
The present application is a divisional application claiming priority under 35 U.S.C. § 121 to U.S. patent application Ser. No. 17/099,139, entitled RADIOISOTOPE ACTIVITY SURVEILLANCE APPARATUS, SYSTEM, AND METHOD, filed Nov. 16, 2020, which is incorporated by reference herein in its respective entirety.
Number | Date | Country | |
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Parent | 17099139 | Nov 2020 | US |
Child | 18792159 | US |