The present application claims priority from Japanese patent application JP 2008-092691 filed on Mar. 31, 2008, the content of which is hereby incorporated by reference into this application.
1. Field of the Invention
The present invention relates to a charged particle beam apparatus, and more particularly to an aberration corrector used in a transmission electron microscope.
2. Background Art
Theoretically, spherical aberrations of electron lenses that use rotationally symmetric electromagnetic fields are always a positive value, and even by compensating for a spherical aberration within a range in which these are used, it is not possible to make the spherical aberration 0. Accordingly, until recently spherical aberration had been the biggest factor limiting the resolution of electron microscope apparatuses.
In contrast, from the latter part of the 1990's, practical application of spherical aberration correctors using non-rotationally symmetric electron optical systems such as multipole lens has been proceeded. Currently, in 2008, at the practical use level, electron microscopes mounted with spherical aberration correctors are been manufactured commercially. In particular, for transmission electron microscopes (TEM) having an accelerating voltage exceeding 100 kV, in many cases the spherical aberration is the biggest factor that determines the resolution, and the effect of utilizing a spherical aberration corrector is significant.
In the process of forming a magnified image, the spherical aberration corrector 2 is arranged directly below the objective lens 4 and compensates for image distortion or blurring that occurs due to a spherical aberration of the objective lens 4. The obtained magnified image is magnified further at a plurality of image-forming lenses 10 that are arranged further downstream, to thereby form an image on an observation surface 11. Normally, a fluorescent screen that is illuminated by the electron beam 8 is arranged on the observation surface, and the magnified image can be observed by viewing this directly. It is also possible to capture an image of the magnified image using a film or CCD camera. In this connection,
In the aforementioned TEM, as a spherical aberration corrector that is appropriate for performing a spherical aberration correction, a configuration including two hexapole lenses that is proposed by H. Rose in JP Patent No. 3207196 (hereunder, referred to as “Patent Document 1”) is currently being practically applied by M. Haider et al.
Although it is known that the hexapole lens 18 has a negative spherical aberration, an aberration such as a three-fold symmetry astigmatic aberration that is unnecessary for correction is also generated at the same time. In such case, it is possible to cancel the three-fold symmetry astigmatic aberration by preparing two of the hexapole lenses 18 and 19 and performing an antisymmetric transfer with the transfer lenses 20 and 21, to thereby extract only a negative spherical aberration (the astigmatic aberration is cancelled by lenses 20 and 21). An adjustment is performed so as to offset the size of the negative spherical aberration with a positive spherical aberration of the objective lens 4 to implement a spherical aberration correction. To establish appropriate transfer conditions, it is necessary to arrange HEX118, HEX219, TL120, and TL221 of the 4f system at the lengths f, 2f, and f as shown in
In contrast, the first half portion is designed to suppress a first off-axis aberration, that is, a coma aberration, which constitutes the next problem after a spherical aberration in a TEM. A coma-free transfer is realized between the objective lens and the 4f system using the two transfer lenses included in the first half portion. Hereunder, the first half portion is referred to as “coma-free plane transfer portion 22”.
A coma-free plane 16 (plane where coma aberration coefficient becomes 0 in polarity inversion process) of the objective lens 4 itself is formed in the vicinity of a back focal plane of the objective lens 4. The coma-free plane 16 of the objective lens 4 is transferred to the center plane of HEX118 as the coma-free plane of the 4f system using the two transfer lenses TF123a and TF224a, to suppress an increase in the coma aberration. In this connection, in order to perform this transfer in a 1:1 ratio, H. Rose stipulates that the lenses in the coma-free plane transfer portion should be disposed at lengths f, 2f, and f as shown in
However, when a condition for disposing lenses in the coma-free plane transfer portion 22 does not comply with the above described 1:1 transfer condition, it is possible to perform a coma-free transfer even outside the restrictive condition of Rose. Conversely, by performing a transfer by imparting a magnification, and not as a 1:1 transfer, there is also the advantage that the effect of the aberration corrector can be adjusted. By focusing on this point, M. Haider et al. disclose a configuration of an improved spherical aberration corrector in JP Patent Publication (Kohyo) No. 2002-510431 B (hereunder, referred to as “Patent Document 2”).
In this connection, in the configuration according to H. Rose shown in
At this time, considering the physical surface of the objective lens, offsetting of a spherical aberration at the spherical aberration corrector and the objective lens is represented by the following expression:
[Expression 2]
c
so+(momt)−4csc=0 (2)
Here, CSO denotes a spherical aberration (coefficient) of the objective lens, CSC denotes a spherical aberration of the spherical aberration corrector, and mO denotes the magnitude of the objective lens. For example, if mt<1 assuming that f1<f2, the spherical aberration CSO of the objective lens 4 can be offset with a smaller correction amount (CSC). Thus, a spherical aberration correction can be adjusted using mt in this manner.
[Non-Patent Document 2] “Upper limits for the residual aberrations of a high-resolution aberration-corrected STEM”, M. Haider, S. Uhlemann, J. Zach, Ultramicroscopy vol. 81, p. 163, (2000)
[Non-Patent Document 2] “Towards sub-0.5 A electron beams”, O. L. Krivanek, P. D. Nellist, N. Dellby, M. F. Murfitt, Z. Szilagyi, Ultramicroscopy vol. 96, p. 229, (2003)
However, with both the configuration according to H. Rose shown in
Further, the problem that fine adjustment is difficult after assembling the apparatus also arises. More specifically, in the case of both H. Rose and M. Haider, because the optical conditions of the coma-free plane transfer portion are fixed once the apparatus configuration has been decided, for example, in a case in which the coma-free plane of the objective lens is displaced from the design position, or when there is no adjustment margin when attempting to change a usage condition of the objective lens such as the magnification or the specimen position from an initial value in accordance with the observation requirements, strictly speaking, the positions of TF1 and TF2 must be shifted in accordance with the displacement from the design values or with the desired optical conditions.
Further, as described in the foregoing, according to the configuration of M. Haider shown in
As described above, in the spherical aberration correctors proposed heretofore, the disposition of lenses is restricted and fixed because of conditions that are necessary for a spherical aberration correction, and thus the degree of freedom in designing a specific apparatus configuration has been limited. Further, after assembling an aberration corrector, the disposition of lenses is fixed and there is no margin left for adjustment. Accordingly in a state in which a corrector is actually being used it is difficult to make an adjustment to the corrector in order to, for example, rectify an error between the design and the manufactured corrector or to correspond to an adjustment according to the actual conditions of use. In particular, since it is difficult to perform a fine adjustment with the 4f system, it is considered that, rather, it is more suitable to use the corrector with fixed conditions. On the other hand, with respect to the coma-free plane transfer portion in the first half of the corrector, it is also considered suitable to provide a flexible adjustment margin with respect to the corrector exterior in order to maintain fixed conditions of the 4f system. For example, as described above, if the transfer magnification mt in the coma-free plane transfer portion 22 can be made variable, by changing mt while keeping the conditions fixed without performing a complicated adjustment of the 4f system such as a hexapole lens adjustment, it is also possible to finely adjust the offsetting between the spherical aberrations of the corrector and the objective lens 4.
The present invention was made in view of the above described circumstances, and an object of the invention is to provide an aberration corrector that has a flexible adjustment margin with respect to the corrector exterior and that guarantees a degree of freedom in the design of a coma-free plane transfer portion even when the mechanical configuration of the aberration corrector has been already decided.
To solve the above described problems, an aberration corrector according to the present invention causes an electron beam trajectory that emanates from a specimen plane (physical surface of an objective lens) to be incident parallel to a multipole lens (HEX118), and causes an electron beam trajectory that emanates from an objective lens coma-free plane or a minimum plane of a fifth-order aberration (center of objective lens) to form an image on a center plane of a multipole lens of the 4f system. As a result, to perform a spherical aberration correction with the 4f system, an antisymmetric transfer is performed between two multipole lenses (HEX118, HEX219), and transfer of a coma-free plane or a minimum plane of a fifth-order aberration is performed to suppress the occurrence of a coma aberration or a fifth-order aberration.
More specifically, an aberration corrector according to the present invention is an aberration corrector for a transmission electron microscope that is disposed downstream of an objective lens of a transmission electron microscope and that performs a spherical aberration correction by offsetting a spherical aberration of the objective lens with a negative spherical aberration that is generated at a combination lens including a plurality of multipole lens, comprising: a spherical aberration correction portion that generates a negative spherical aberration; and a transfer portion that is provided between the objective lens and the spherical aberration correction portion and that has a first and a second spherical transfer lens that suppress an occurrence of a coma aberration or a fifth-order aberration. The transfer portion transfers a coma-free plane or a minimum plane of a fifth-order aberration of the objective lens that is formed in the vicinity of a back focal plane of the objective lens to a coma-free plane of the spherical aberration correction portion or a center plane of a first lens (multipole lens located at an upstream position) of the spherical aberration correction portion, and causes an electron beam that is scattered at a specimen and emanates from a specimen plane to be incident in parallel with the spherical aberration correction portion. Further, among the two spherical transfer lenses of the coma-free plane transfer portion, a length between the objective lens and the first spherical transfer lens that is arranged at a nearest position to the objective lens is different to a focal length of the first spherical transfer lens.
Further, an aberration corrector according to the present invention is an aberration corrector for a transmission electron microscope that is disposed downstream of an objective lens of a transmission electron microscope and that performs a spherical aberration correction by offsetting a spherical aberration of the objective lens with a negative spherical aberration that is generated at a combination lens including a plurality of multipole lens, comprising: a spherical aberration correction portion that generates a negative spherical aberration; and a transfer portion that is provided between the objective lens and the spherical aberration correction portion and that has a first, a second, and a third spherical transfer lens that suppress an occurrence of a coma aberration or a fifth-order aberration, and that enables an adjustment of a transfer magnification to the spherical aberration correction portion from the objective lens by means of the spherical transfer lenses. The transfer portion transfers a coma-free plane or a minimum plane of a fifth-order aberration of the objective lens that is formed in the vicinity of a back focal plane of the objective lens to a coma-free plane of the spherical aberration correction portion or a center plane of a first lens (multipole lens located at an upstream position) of the spherical aberration correction portion, and causes an electron beam that is scattered at a specimen and emanates from a specimen plane to be incident in parallel with the spherical aberration correction portion. Further, among the three spherical transfer lenses of the transfer portion, a length between the objective lens and the first spherical transfer lens that is arranged at a nearest position to the objective lens is different to a focal length of the first spherical transfer lens.
Other features of the present invention will be apparent from the preferred embodiments of the invention that are described below and from the attached drawings.
According to the present invention, it is possible to guarantee a degree of freedom in the design of a coma-free plane transfer portion even when the mechanical configuration of an aberration corrector has been already decided, and to provide a flexible adjustment margin with respect to the corrector exterior.
An object of the present invention is to improve the resolution in a charged particle beam apparatus. In particular, the present invention relates to an apparatus that compensates for a spherical aberration in a transmission electron microscope. Similarly to the prior art, an aberration corrector according to the present invention can be applied to the charged particle beam apparatus (transmission electron microscope apparatus) shown in
Hereunder, embodiments of the present invention are described with reference to the attached drawings. However, the following embodiments are merely examples for implementing the present invention, and it should be noted that these embodiments do not limit the technical scope of the present invention. Common components are denoted by the same reference numerals in the drawings.
First, the principles of the present invention will be described.
The lens configuration of a coma-free plane transfer portion that can provide an adjustment margin in order to, for example, rectify an error between a design and a manufactured corrector or to correspond to an adjustment according to actual usage conditions while maintaining the coma-free plane transfer conditions is described below. First, the coma-free plane transfer conditions are compiled below.
Condition 1: An electron beam trajectory 13 emanating from a specimen plane (physical surface of objective lens) is caused to be incident in parallel with the HEX118. (The electron beam trajectory in question corresponds to the trajectory of an electron beam that is scattered from the specimen. This is a necessary condition for performing an antisymmetric transfer between the HEX118 and the HEX219 in order to perform a spherical aberration correction in a 4f system 17).
Condition 2: An electron beam trajectory 14 emanating from an objective-lens coma-free plane 16 forms an image on a 4f-system coma-free plane (center plane of HEX118). (This is a necessary condition for performing a coma-free transfer to suppress the generation of a coma aberration.)
Here, l1, l2, and l3 denote lengths between the objective lens and TF1, TF1 and TF2, and TF2 and HEX1, respectively, as shown in each drawing. Further, f1, and f2 denote the focal lengths of TF123c and TF224c, respectively. b2 denotes a length from the relevant lens as far as a plane at which the TF224c transfers the coma-free plane 16, taking the electron trajectory of condition 2 into consideration, and is represented by the following relation based on the formula of the lens using the aforementioned l1, l2, and l3, and f1 and f2.
Provided, b1 denotes a length from the TF123c to an intermediate transfer plane of the coma-free plane.
By combining expression 3, expression 4, and expression 5 to solve f1 and f2, expression 6 is established.
Provided, Lt is the entire length of the coma-free plane transfer portion 22, that is, expression 7.
[Expression 7]
L
t
=l
1
+l
2
+l
3 (7)
Further, K is a parameter represented by expression 8 below
[Expression 8]
K=√{square root over (l22−4l1l3)} (8)
That is, the solution represented by expression 6 is a real solution in a range in which K is a real number, that is, in a case in which expression 9 is satisfied.
[Expression 9]
l2>2√{square root over (l1l3)} (9)
Naturally, l1, l2, and l3 are positive numbers, and in a range in which expression 9 has a solution with a simple operation, f1 and f2 of expression 6 can also be shown to be positive values.
The foregoing description shows that, while satisfying conditions relating to the coma-free plane transfer portion 22 of conditions 1 and 2, focal lengths f1 and f2 of the TF1 and TF2 that are effective for arbitrary lens intervals 11, 12, and 13 can be found within a range in which expression 9 has a solution. This result remarkably increases the degree of freedom with respect to the disposition of lenses in the coma-free plane transfer portion at the design stage, and further, after the disposition of lenses has been fixed, it is possible to perform a fine adjustment according to expression 6 even in an operating state.
The addition of a third transfer lens may also be considered to give the coma-free plane transfer portion 22 an adjustable magnification. Using the increased flexibility obtained by addition of a lens, leeway is generated that makes it possible to control the transfer magnification of the coma-free plane transfer portion 22 while maintaining the coma-free plane transfer conditions.
Next, a specific example is given and examined based on the above described principles of the invention. In this case, regarding the configuration shown in
[Expression 10]
l2>30√{square root over (6)}≈73.5 mm (10)
When l2 is a value in the range shown by expression 10, the coma-free plane transfer portion 22 has a solution according to expression 6 that establishes the aforementioned conditions 1 and 2. In this connection, expression 10 is, for example, represented with an accuracy of ±1%.
A graph 25 shown in
In contrast, as shown in a graph 26 in
In this connection, a case in which it is assumed that l2=l1+l3=75 mm under the condition shown in the graph is equivalent to the spherical aberration corrector according to M. Haider (see
Thus, according to the present invention, the condition (l2=l1+l3, l1=l3=l2/2) should be omitted from expression 6, and is summarized as l1≠f1, l3≠f2.
As described in the foregoing, since adjustment of the 4f system is difficult, it is desirable that execution of a fine adjustment of a spherical aberration correction is concentrated on transfer lenses of a coma-free plane transfer portion while maintaining the 4f system in a fixed condition. To achieve this, a three-lens configuration is adopted by adding a single lens TF324d the transfer lenses that had been a two-lens configuration comprising TF1 and TF2. It is thereby possible to vary the transfer magnification mt in a zooming manner while maintaining the coma-free transfer conditions. That is, the degree of freedom in setting a transfer magnification can also be increased.
According to the second embodiment, as shown in
Provided, it is assumed that the lengths between the objective lens 4 and TF127, TF127 and TF223d, TF223d and TF324d, and TF324d and HEX118, are l1, l2, l3, and l4, respectively, and the second term in each expression is given as follows taking l1≡L as a reference.
[Expression 12]
l1≡L
l2=k2L
l3=k3L
l4=k4L (12)
As shown in expression 11, since mt can be left as an independent variable, it is possible to adjust the transfer magnification mt while maintaining the coma-free transfer conditions. Further, when each of the lenses are arranged at regular intervals (that is, when l1=l2=l3=l4=≡L), f1, f2, and f3 are given by expression 13.
According to expression 13, a positive number solution can be found for f1, f2, and f3 when mt<0. As an example, the relation when L=30 mm (expression 13) is plotted in a graph 28 of
Provided, when it is assumed that mt≡δmt−1, and O(δm2) is a term that is equal to or greater than the square of δm, the influence when δm<<⅘ is small. Accordingly, as an adjustment operation when δm is in the above range, first, in order to obtain mt=−1, expression 15 is taken as the reference state.
[Expression 15]
f1=L/2
f
2
=L/4
f
3
=L/2 (15)
Since f2 changes only in the second order or higher with respect to δm, it is found that it is sufficient that f1 and f3 are deflected to their respective antisymmetries for every δm/4 at TF123d and TF327 while TF224d remains fixed. Thus, by applying a condition (arranging lenses at regular intervals) to expression 13 to simplify the expression so as to obtain expression 14, the adjustment operation is simplified.
The electron beam trajectory in the reference state that results in mt=−1 is shown in the drawing denoted by reference number 29 in
Provided, in Table 1, t1 and t2 are the lengths from the respective lenses to a plane at which the transfer lenses TF1 and TF2 respectively transfer the coma-free plane.
As described in the foregoing, with respect to the configuration of transfer lenses in a coma-free plane transfer portion, the present invention enables flexible arrangement and electro-optic fine adjustment with a two-lens system. Further, when using three lenses, the present invention provides means that adjusts a spherical aberration correction strength while keeping the 4f system fixed and with a transfer magnification independent thereof.
In this connection, although restrictive conditions of the transfer lens portion are described with respect to a coma-free transfer in the above description, the present invention can also be applied under a condition which transfers two similar specific planes (planes limited by a specimen plane and a transfer condition; the coma-free plane in the above description). Conditions other than a coma-free plane transfer include, for example, minimization of a fifth-order spherical aberration. In this case, it is sufficient to consider a transfer by substituting a plane that serves as a minimum plane of a fifth-order aberration (for example, center of objective lens) for the coma-free plane in the above description.
As the spherical aberration correction portion in the above description, a spherical aberration correction portion that uses hexapole lenses based on the configurations of H. Rose and M. Haider is described. However, it is also possible to provide a spherical aberration correction portion that uses other multi-stage multipole lenses instead of using hexapole lenses. In this case also, the consideration for transferring an image from the objective lens to the spherical aberration correction portion with specific restrictive conditions is the same, and it is also the same that the adjustment of a transfer lens portion comprising an ordinary spherical lens is easier than adjustment of a spherical aberration correction portion comprising multiple poles. The conditions in this case are also the same as in the case of hexapole lenses.
Number | Date | Country | Kind |
---|---|---|---|
2008-092691 | Mar 2008 | JP | national |